Chen Xueer, Zhang Yong, Cai Guoxiong, Zhuo Jianliang, Lai Kunzhong, Ye Longfang
Institute of Electromagnetics and Acoustics, School of Electronic Science and Engineering, Xiamen University, Xiamen 361005, China.
Shenzhen Research Institute of Xiamen University, Shenzhen 518057, China.
Nanophotonics. 2022 Sep 19;11(20):4537-4549. doi: 10.1515/nanoph-2022-0394. eCollection 2022 Sep.
We propose and numerically demonstrate high Q-factor sensors based on all-dielectric metasurfaces, which are very sensitive to the change of the refractive index of the surrounding media and the incident angle. By using the light incident angular scanning method, the all-dielectric metasurface based on symmetric tetramer can act as an excellent sensing platform for trace-amount molecules such as protein A/G, 2, 4-DNT, and 2D material graphene with huge absorbance enhancement in the mid-infrared broadband spectrums. The results reveal that envelope of absorbance amplitudes is in good agreement with the vibrational mode of molecules, and absorbance enhancement factors reach as high as 10 dB in the mid-infrared wavelength range from 5.75 to 6.80 μm. To further increase the Q-factor of the resonances, the all-dielectric metasurface based on asymmetric tetramer is investigated. This asymmetric structure can induce toroidal and magnetic dipoles governed by quasi-BIC to produce multi-extremely narrow linewidth Fano resonances, and the maximum sensitivity reaches up to 1.43 μm/RIU. Therefore, the proposed all-dielectric metasurface demonstrates highly enhanced performance in refractive index and chemical information sensing for trace-amount biomolecules, which inspires the development of new high-sensitivity refractive index sensors for the nondestructive identification in the mid-infrared regime.
我们提出并通过数值模拟证明了基于全介质超表面的高Q因子传感器,该传感器对周围介质的折射率变化和入射角非常敏感。通过使用光入射角度扫描方法,基于对称四聚体的全介质超表面可以作为一个出色的传感平台,用于检测诸如蛋白A/G、2,4-二硝基甲苯和二维材料石墨烯等痕量分子,在中红外宽带光谱中具有巨大的吸光度增强。结果表明,吸光度振幅包络与分子的振动模式高度吻合,在5.75至6.80μm的中红外波长范围内,吸光度增强因子高达10dB。为了进一步提高共振的Q因子,我们研究了基于不对称四聚体的全介质超表面。这种不对称结构可以诱导由准束缚态诱导产生的环形和磁偶极子,以产生多极极窄线宽的法诺共振,最大灵敏度高达1.43μm/RIU。因此,所提出的全介质超表面在痕量生物分子的折射率和化学信息传感方面表现出高度增强的性能,这为在中红外区域进行无损识别的新型高灵敏度折射率传感器的开发提供了启示。