Mičica Martin, Wright Adrien, Koleják Pierre, Lezier Geoffrey, Postava Kamil, Hawecker Jacques, De Vetter Anna, Tignon Jerome, Mangeney Juliette, Jaffres Henri, Lebrun Romain, Tiercelin Nicolas, Vanwolleghem Mathias, Dhillon Sukhdeep
Laboratoire de Physique de l'Ecole Normale Supérieure, ENS, Université PSL, CNRS, Sorbonne Université, Université Paris Cité, F-75005, Paris, France.
Univ. Lille, CNRS, Centrale Lille, Univ. Polytechnique Hauts-de-France, UMR 8520-IEMN, F-59000, Lille, France.
Nanophotonics. 2024 Mar 1;13(10):1899-1907. doi: 10.1515/nanoph-2023-0807. eCollection 2024 Apr.
Spintronic terahertz emitters (STEs), based on optical excitation of nanometer thick ferromagnetic/heavy metal (FM/HM) heterojunctions, have become important sources for the generation of terahertz (THz) pulses. However, the efficiency of the optical-to-THz conversion remains limited. Although optical techniques have been developed to enhance the optical absorption, no investigations have studied the application of THz cavities. Here, to enhance the THz efficiency of STEs in a selected THz spectral range, FM/HM structures are realized on ultra-thin sapphire layers with metallic mirrors to create /4 THz resonant cavities. THz emission time domain spectroscopy of these STE/sapphire/mirror heterostructures, with sapphire thicknesses ranging from 110 µm to 25 µm, shows enhancement of the emitted THz field that fits the /4 cavity resonance with up to a doubling of the field in the spectrum, and in agreement with temporal simulations of the emitted THz pulse. By taking advantage of birefringent materials, we further show the potential of control of the polarization state of the emitted THz pulse. This work shows the potential of enhancing and engineering THz emission from STEs using THz cavities that can be controlled over a broad spectral range, which can be easily combined with optical cavities.
基于纳米厚铁磁/重金属(FM/HM)异质结光激发的自旋电子太赫兹发射器(STE)已成为太赫兹(THz)脉冲产生的重要源。然而,光到太赫兹的转换效率仍然有限。尽管已经开发了光学技术来增强光吸收,但尚未有研究探讨太赫兹腔的应用。在此,为了在选定的太赫兹光谱范围内提高STE的太赫兹效率,在具有金属镜的超薄蓝宝石层上实现FM/HM结构,以创建λ/4太赫兹谐振腔。对这些STE/蓝宝石/镜异质结构进行太赫兹发射时域光谱分析,蓝宝石厚度范围为110μm至25μm,结果表明发射的太赫兹场增强,符合λ/4腔共振,光谱中的场强最多可翻倍,并且与发射的太赫兹脉冲的时间模拟结果一致。通过利用双折射材料,我们进一步展示了控制发射太赫兹脉冲偏振态的潜力。这项工作展示了利用太赫兹腔增强和调控STE太赫兹发射的潜力,该太赫兹腔可在很宽的光谱范围内进行控制,并且能够轻松地与光学腔相结合。