Li Chao, Lu Yan, Li Ruoning, Wang Li, Weismann Alexander, Berndt Richard
Institut für Experimentelle und Angewandte Physik, Christian-Albrechts-Universität, 24098 Kiel, Germany.
Department of Physics, Nanchang University, Nanchang 330031, People's Republic of China.
Nano Lett. 2025 Jan 29;25(4):1504-1511. doi: 10.1021/acs.nanolett.4c05409. Epub 2025 Jan 13.
The mechanical coupling between molecules represents a promising route for the development of molecular machines. Constructing molecular gears requires easily rotatable and mutually interlocked pinions. Using scanning tunneling microscopy (STM), it is demonstrated that aluminum phthalocyanine (AlPc) molecules on Pb(100) exhibit these properties. Unlike other phthalocyanines on this substrate, isolated AlPc molecules fluctuate between two azimuthal orientations. Density functional theory (DFT) calculations confirm two stable orientations of single molecules and indicate a relatively low rotation barrier. In STM-constructed dimers and trimers, fluctuations diminish, and various molecular orientations are stabilized. Induced collective rotation of all molecules in the trimers is observed, demonstrating their mechanical interlocking. Potential functions describing angle and distance dependencies of intermolecular and molecule-substrate interactions are derived from DFT calculations of dimers; 52 experimentally determined trimer geometries are reproduced using these potentials. This intuitive approach may prove to be useful in modeling larger structures beyond the scope of quantum mechanical descriptions.
分子间的机械耦合是分子机器发展的一条很有前景的途径。构建分子齿轮需要易于旋转且相互联锁的小齿轮。利用扫描隧道显微镜(STM)表明,Pb(100)上的铝酞菁(AlPc)分子具有这些特性。与该衬底上的其他酞菁不同,孤立的AlPc分子在两个方位取向之间波动。密度泛函理论(DFT)计算证实了单分子的两个稳定取向,并表明旋转势垒相对较低。在STM构建的二聚体和三聚体中,波动减小,各种分子取向得以稳定。观察到三聚体中所有分子的诱导集体旋转,证明了它们的机械联锁。描述分子间和分子 - 衬底相互作用的角度和距离依赖性的势函数来自二聚体的DFT计算;使用这些势函数再现了52个实验确定的三聚体几何结构。这种直观的方法可能被证明在对超出量子力学描述范围的更大结构进行建模时是有用的。