Mauri Giacomo, Sykora G Jeff, Smith Gregory N, Parnell Steven R, Dalgliesh Robert M, Honecker Dirk, Mann Sarah E, Schooneveld Erik M, Rhodes Nigel J
Science and Technology Facilities Council, ISIS Neutron and Muon Source, Rutherford Appleton Laboratory, Didcot, Oxfordshire, OX11 0QX, UK.
Sci Rep. 2025 Jan 31;15(1):3877. doi: 10.1038/s41598-025-87864-1.
Neutron spin-echo techniques exploit Larmor precession of the neutron spin to encode either the scattering angle or energy. These are powerful means to extend the measurable momentum transfer (Q) and energy (E) range in neutron scattering measurements. Standard small-angle neutron scattering (SANS) instruments are sensitive in a range of 10-200 nm, whereas these techniques allow the study of structures in materials on length scales of tens of nm up to tens of m. The Larmor instrument at ISIS is equipped to operate in spin-echo modulated SANS (SEMSANS) and spin-echo SANS (SESANS) mode. Two separate detectors were developed to cope with the performance demands set by these techniques. The first is a position sensitive ZnS:Ag/LiF scintillator-based detector coupled with wavelength shifting fibres that can be used for both SEMSANS and SESANS. A detector prototype using GS20 glass scintillator directly coupled to a multi-anode photomultiplier was developed as an alternative for SESANS measurements at higher incident neutron fluxes. The designs and results obtained with the two detectors are presented together with future improvements to both technologies. These, in addition to promising development routes, demonstrate the potential for utilising a WLSF ZnS:Ag/LiF scintillator detector and a pixelated GS20 detector for SEMSANS and SESANS applications.
中子自旋回波技术利用中子自旋的拉莫尔进动来编码散射角或能量。这些是在中子散射测量中扩展可测量动量转移(Q)和能量(E)范围的有力手段。标准小角中子散射(SANS)仪器在10 - 200纳米范围内敏感,而这些技术允许研究材料中长度尺度从几十纳米到几十微米的结构。ISIS的拉莫尔仪器配备了以自旋回波调制SANS(SEMSANS)和自旋回波SANS(SESANS)模式运行的装置。开发了两个独立的探测器来满足这些技术提出的性能要求。第一个是基于位置敏感的ZnS:Ag/LiF闪烁体的探测器,与波长移位光纤耦合,可用于SEMSANS和SESANS。开发了一种使用直接耦合到多阳极光电倍增管的GS20玻璃闪烁体的探测器原型,作为在更高入射中子通量下进行SESANS测量的替代方案。介绍了两种探测器的设计和结果以及对这两种技术的未来改进。这些,除了有前景的发展路线外,还展示了将WLSF ZnS:Ag/LiF闪烁体探测器和像素化GS20探测器用于SEMSANS和SESANS应用的潜力。