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使用ZnS:Ag/LiF和锂玻璃闪烁体的自旋回波小角中子散射技术的探测器开发。

Detector development for spin-echo SANS techniques using ZnS:Ag/LiF and Li glass scintillators.

作者信息

Mauri Giacomo, Sykora G Jeff, Smith Gregory N, Parnell Steven R, Dalgliesh Robert M, Honecker Dirk, Mann Sarah E, Schooneveld Erik M, Rhodes Nigel J

机构信息

Science and Technology Facilities Council, ISIS Neutron and Muon Source, Rutherford Appleton Laboratory, Didcot, Oxfordshire, OX11 0QX, UK.

出版信息

Sci Rep. 2025 Jan 31;15(1):3877. doi: 10.1038/s41598-025-87864-1.

DOI:10.1038/s41598-025-87864-1
PMID:39890987
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11785970/
Abstract

Neutron spin-echo techniques exploit Larmor precession of the neutron spin to encode either the scattering angle or energy. These are powerful means to extend the measurable momentum transfer (Q) and energy (E) range in neutron scattering measurements. Standard small-angle neutron scattering (SANS) instruments are sensitive in a range of  10-200 nm, whereas these techniques allow the study of structures in materials on length scales of tens of nm up to tens of m. The Larmor instrument at ISIS is equipped to operate in spin-echo modulated SANS (SEMSANS) and spin-echo SANS (SESANS) mode. Two separate detectors were developed to cope with the performance demands set by these techniques. The first is a position sensitive ZnS:Ag/LiF scintillator-based detector coupled with wavelength shifting fibres that can be used for both SEMSANS and SESANS. A detector prototype using GS20 glass scintillator directly coupled to a multi-anode photomultiplier was developed as an alternative for SESANS measurements at higher incident neutron fluxes. The designs and results obtained with the two detectors are presented together with future improvements to both technologies. These, in addition to promising development routes, demonstrate the potential for utilising a WLSF ZnS:Ag/LiF scintillator detector and a pixelated GS20 detector for SEMSANS and SESANS applications.

摘要

中子自旋回波技术利用中子自旋的拉莫尔进动来编码散射角或能量。这些是在中子散射测量中扩展可测量动量转移(Q)和能量(E)范围的有力手段。标准小角中子散射(SANS)仪器在10 - 200纳米范围内敏感,而这些技术允许研究材料中长度尺度从几十纳米到几十微米的结构。ISIS的拉莫尔仪器配备了以自旋回波调制SANS(SEMSANS)和自旋回波SANS(SESANS)模式运行的装置。开发了两个独立的探测器来满足这些技术提出的性能要求。第一个是基于位置敏感的ZnS:Ag/LiF闪烁体的探测器,与波长移位光纤耦合,可用于SEMSANS和SESANS。开发了一种使用直接耦合到多阳极光电倍增管的GS20玻璃闪烁体的探测器原型,作为在更高入射中子通量下进行SESANS测量的替代方案。介绍了两种探测器的设计和结果以及对这两种技术的未来改进。这些,除了有前景的发展路线外,还展示了将WLSF ZnS:Ag/LiF闪烁体探测器和像素化GS20探测器用于SEMSANS和SESANS应用的潜力。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b674/11785970/b8357f58369c/41598_2025_87864_Fig7_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b674/11785970/0b0b700f0d08/41598_2025_87864_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b674/11785970/0f1fe1f2985e/41598_2025_87864_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b674/11785970/da82e225ae11/41598_2025_87864_Fig6_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b674/11785970/b8357f58369c/41598_2025_87864_Fig7_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b674/11785970/0b0b700f0d08/41598_2025_87864_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b674/11785970/0f1fe1f2985e/41598_2025_87864_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b674/11785970/da82e225ae11/41598_2025_87864_Fig6_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b674/11785970/b8357f58369c/41598_2025_87864_Fig7_HTML.jpg

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本文引用的文献

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2
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Rev Sci Instrum. 2024 Mar 1;95(3). doi: 10.1063/5.0189920.
3
Unveiling contextual realities by microscopically entangling a neutron.
通过微观纠缠一个中子来揭示背景现实。
Nat Commun. 2020 Feb 18;11(1):930. doi: 10.1038/s41467-020-14741-y.
4
Time of flight modulation of intensity by zero effort on Larmor.通过对拉莫尔频率零努力实现强度的飞行时间调制。
Rev Sci Instrum. 2019 Dec 1;90(12):125101. doi: 10.1063/1.5123987.
5
Data Correction of Intensity Modulated Small Angle Scattering.强度调制小角散射的数据校正
Sci Rep. 2019 Jun 12;9(1):8563. doi: 10.1038/s41598-019-44493-9.
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Improved neutron-gamma discrimination for a (6)Li-glass neutron detector using digital signal analysis methods.使用数字信号分析方法改进用于(6)锂玻璃中子探测器的中子-伽马甄别能力。
Rev Sci Instrum. 2016 Jan;87(1):013301. doi: 10.1063/1.4939821.
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Spin echo small angle neutron scattering using a continuously pumped (3)He neutron polarisation analyser.使用连续抽运的³He中子极化分析仪的自旋回波小角中子散射
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Development of a neutron detector based on a position-sensitive photomultiplier.基于位置灵敏光电倍增管的中子探测器的研制。
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