Bömeke Paul, Petersen Maike
Institut für Pharmazeutische Biologie und Biotechnologie, Philipps-Universität Marburg, Robert-Koch-Str. 4, Marburg, 35037, Germany.
Plant J. 2025 Mar;121(5):e70035. doi: 10.1111/tpj.70035.
Sarcandra glabra (Chloranthaceae) has an elaborate phenolic metabolism, encompassing various hydroxycinnamic acid esters. This may imply that multiple hydroxycinnamoyltransferases are involved in establishing this spectrum of natural compounds. Five coding sequences from S. glabra, belonging to the superfamily of BAHD acyltransferases, have been amplified from S. glabra cDNA, and the proteins were expressed in Escherichia coli. By assaying the proteins biochemically, the main substrates of these enzymes were identified as p-coumaroyl- and caffeoyl-CoA as donor substrates together with varying acceptor substrates. SgHST mainly forms p-coumaroyl- and caffeoylshikimic acid, but also the corresponding quinic acid esters as well as amides with 3- and 5-hydroxyanthranilic acids. SgHQT1 predominantly catalyzes the formation of p-coumaroyl- and caffeoyl-5-O-quinic acid, while SgHQT2 correspondingly forms p-coumaroyl- and caffeoyl-4-O-quinic acid. To our knowledge, this is the first characterized enzyme forming cryptochlorogenic acid and its precursor p-coumaroyl-4-O-quinic acid. SgRAS synthesizes rosmarinic acid and its precursors (caffeoyl-4'-hydroxyphenyllactic, p-coumaroyl-4'-hydroxyphenyllactic, p-coumaroyl-3',4'-dihydroxyphenyllactic acids) as well as amides with aromatic d-amino acids. No substrates could be identified for the fifth sequence, SgHCT-F, which phylogenetically groups with benzyl alcohol O-benzoyltransferases. All enzymes, except SgHCT-F, were fully kinetically characterized, and their expression in different tissues of S. glabra was assessed.
肿节风(金粟兰科)具有复杂的酚类代谢,包括多种羟基肉桂酸酯。这可能意味着多种羟基肉桂酰转移酶参与了这类天然化合物的合成。从肿节风cDNA中扩增出了5个属于BAHD酰基转移酶超家族的编码序列,并在大肠杆菌中表达了相应的蛋白质。通过对这些蛋白质进行生化分析,确定了这些酶的主要供体底物为对香豆酰辅酶A和咖啡酰辅酶A,同时还有不同的受体底物。SgHST主要形成对香豆酰和咖啡酰莽草酸,还能形成相应的奎尼酸酯以及与3-和5-羟基邻氨基苯甲酸的酰胺。SgHQT1主要催化形成对香豆酰和咖啡酰-5-O-奎尼酸,而SgHQT2相应地形成对香豆酰和咖啡酰-4-O-奎尼酸。据我们所知,这是首次鉴定出形成隐绿原酸及其前体对香豆酰-4-O-奎尼酸的酶。SgRAS合成迷迭香酸及其前体(咖啡酰-4'-羟基苯乳酸、对香豆酰-4'-羟基苯乳酸、对香豆酰-3',4'-二羟基苯乳酸)以及与芳香族D-氨基酸的酰胺。对于第五个序列SgHCT-F,未鉴定出底物,该序列在系统发育上与苄醇O-苯甲酰转移酶归为一类。除SgHCT-F外,对所有酶都进行了完整的动力学表征,并评估了它们在肿节风不同组织中的表达情况。