Suryanarayana M V
Bhabha Atomic Research Centre, Visakhapatnam, Andhra Pradesh, India.
Sci Rep. 2025 Mar 27;15(1):10543. doi: 10.1038/s41598-024-80936-8.
This present study investigates a three-step laser isotope separation method for the enrichment of Er isotope using 631.052 nm - 586.912 nm - 566.003 nm three-step photoionization scheme. The lineshape contours observed in three-step photoionization process have been investigated in detail. This study shows that enrichment of Er isotope can be achieved with a relatively simple experimental configuration. With the derived system configuration, it has been shown that it is possible to produce 18 g/day of 90% enriched Er. Using the enriched Er isotope obtained from the laser isotope separation process, irradiation in low, medium, and high flux reactors can produce 180, 1800, and 18,000 doses per day (each with an activity of 7.4 GBq) respectively. After 24 h of irradiation and chemical separation, the radioisotopic purity of the medical isotope reaches to > 99% making it suitable for the medical applications. This is the first ever study on the laser isotope separation of Er isotope.
本研究探讨了一种三步激光同位素分离方法,用于使用631.052纳米 - 586.912纳米 - 566.003纳米三步光电离方案富集铒同位素。详细研究了三步光电离过程中观察到的线形轮廓。本研究表明,通过相对简单的实验配置即可实现铒同位素的富集。利用推导的系统配置,已证明每天可生产18克90%富集度的铒。使用从激光同位素分离过程中获得的富集铒同位素,在低通量、中通量和高通量反应堆中辐照,每天可分别产生180、1800和18000剂(每剂活度为7.4吉贝可)。辐照24小时并经过化学分离后,医用同位素的放射性纯度达到>99%,使其适用于医学应用。这是首次关于铒同位素激光同位素分离的研究。