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磁性 Kagome 材料:连接基本性质与拓扑量子应用

Magnetic Kagome materials: bridging fundamental properties and topological quantum applications.

作者信息

Negi Pranav, Medhi Koushik, Pancholi Abhinav, Roychowdhury Subhajit

机构信息

Department of Chemistry, Indian Institute of Science Education and Research Bhopal, Bhopal-462 066, India.

出版信息

Mater Horiz. 2025 Jun 30;12(13):4510-4544. doi: 10.1039/d5mh00120j.

Abstract

Kagome materials, characterized by their unique lattice structure and electronic properties such as Dirac cones, flat bands, van Hove singularities, and topologically nontrivial surface states, have become a focal point in solid state chemistry and condensed matter physics. The combination of spin-orbit coupling (SOC) and magnetism in these materials leads to several notable phenomena, such as the large anomalous Hall effect and anomalous Nernst effect observed in noncollinear antiferromagnets like MnSn and MnGe and Weyl semimetal behaviour in CoSnS. The interplay between charge order, superconductivity, and symmetry breaking in materials like AVSb, LaRuSi, and CeRu unveils a rich landscape of emergent quantum phenomena, in addition to the distorted Kagome lattice in HoAgGe, along with the flat band, saddle point, and Dirac cones in YMnSn. Topological skyrmions in FeGe and the quantum Chern insulating phase in TbMnSn further underscore the rich physics of these materials. Therefore, Kagome materials are uniquely suited to study the interaction between topology, magnetism, and electron correlation. This review comprehensively covers the progress in topological Kagome magnets, the fundamental concepts, and the connections between their exotic properties and the Kagome lattice structure. In conclusion, several open questions and future research directions are highlighted, providing valuable insights for researchers aiming to advance this integrated field. This review serves as a reference for understanding the potential of Kagome materials and their future advancements, fostering further exploration of their complex and promising properties.

摘要

戈薇材料以其独特的晶格结构和电子特性(如狄拉克锥、平带、范霍夫奇点和拓扑非平凡表面态)而著称,已成为固态化学和凝聚态物理的焦点。这些材料中自旋轨道耦合(SOC)和磁性的结合导致了几种显著现象,例如在MnSn和MnGe等非共线反铁磁体中观察到的大反常霍尔效应和反常能斯特效应,以及CoSnS中的外尔半金属行为。在AVSb、LaRuSi和CeRu等材料中,电荷序、超导性和对称性破缺之间的相互作用揭示了丰富的涌现量子现象景观,此外还有HoAgGe中扭曲的戈薇晶格,以及YMnSn中的平带、鞍点和狄拉克锥。FeGe中的拓扑斯格明子和TbMnSn中的量子陈绝缘相进一步突出了这些材料丰富的物理性质。因此,戈薇材料特别适合研究拓扑、磁性和电子关联之间的相互作用。本综述全面涵盖了拓扑戈薇磁体的进展、基本概念,以及它们的奇异性质与戈薇晶格结构之间的联系。最后,强调了几个悬而未决的问题和未来的研究方向,为旨在推进这一综合领域的研究人员提供了有价值的见解。本综述作为理解戈薇材料潜力及其未来进展的参考,促进了对其复杂且有前景的性质的进一步探索。

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