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多孔稠合芳香网络及其应用的最新进展

Recent Progress in Porous Fused Aromatic Networks and Their Applications.

作者信息

Ahmad Ishfaq, Mahmood Javeed, Baek Jong-Beom

机构信息

School of Energy and Chemical Engineering/Center for Dimension-Controllable Organic Frameworks Ulsan National Institute of Science and Technology (UNIST) UNIST 50 Ulsan 44919 Republic of Korea.

出版信息

Small Sci. 2020 Oct 21;1(1):2000007. doi: 10.1002/smsc.202000007. eCollection 2021 Jan.

DOI:10.1002/smsc.202000007
PMID:40212411
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11935964/
Abstract

Porous materials are ubiquitous in nature and play central roles in ecosystems and human life. Porous fused aromatic networks (P-FANs) are emerging as a new class of porous organic materials, which can be precisely constructed from organic precursors via the formation of irreversible fused aromatic rings. Despite the luculent advantages offered by P-FANs, the research community has conventionally focused on more synthetically accessible covalent organic frameworks (COFs), which mostly involve reversible condensation reactions. An overview of the trend in the field of P-FANs and their possible applications in different fields, including proton conduction, catalysis, gas storage, supercapacitors, and optoelectronics, is presented herein.

摘要

多孔材料在自然界中无处不在，在生态系统和人类生活中发挥着核心作用。多孔稠合芳环网络（P-FANs）正作为一类新型的多孔有机材料崭露头角，它可以通过不可逆稠合芳环的形成由有机前体精确构建而成。尽管P-FANs具有明显的优势，但传统上研究界更多地关注合成上更容易获得的共价有机框架（COFs），其大多涉及可逆缩合反应。本文概述了P-FANs领域的发展趋势及其在不同领域的可能应用，包括质子传导、催化、气体存储、超级电容器和光电子学。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a9d3/11935964/10795c30c602/SMSC-1-2000007-g011.jpg
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https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a9d3/11935964/124d78dc6acb/SMSC-1-2000007-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a9d3/11935964/e895e44d4f2c/SMSC-1-2000007-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a9d3/11935964/771e18a99b63/SMSC-1-2000007-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a9d3/11935964/d21e09b166cc/SMSC-1-2000007-g013.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a9d3/11935964/e885664e0198/SMSC-1-2000007-g007.jpg
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本文引用的文献

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Covalent Organic Frameworks: Design, Synthesis, and Functions.共价有机框架：设计、合成与功能。
Chem Rev. 2020 Aug 26;120(16):8814-8933. doi: 10.1021/acs.chemrev.9b00550. Epub 2020 Jan 22.
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Unveiling Electronic Properties in Metal-Phthalocyanine-Based Pyrazine-Linked Conjugated Two-Dimensional Covalent Organic Frameworks.揭示基于金属酞菁的吡嗪连接共轭二维共价有机框架中的电子性质
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