Huang Yifei, Deng Yujun, Yi Peiyun, Peng Linfa
Shanghai Key Laboratory of Digital Manufacture for Thin-Walled Structures, Shanghai Jiao Tong University, Shanghai 200240, P. R. China.
State Key Laboratory of Mechanical System and Vibration, Shanghai Jiao Tong University, Shanghai 200240, P. R. China.
ACS Appl Mater Interfaces. 2025 Apr 30;17(17):25839-25848. doi: 10.1021/acsami.5c04159. Epub 2025 Apr 19.
Stretchable electronics face the challenge of long-term stable operation, and one of the difficulties is that the core component electrodes maintain a high conductivity under multiple stretchable deformations. To address this issue, we propose a highly fatigue-resistant stretchable metal film electrode, which consists of a platinum nanofilm prebent into regular microconvex stripes on the surface of an elastomeric material. The electrical conductivity of the stretchable electrode is 4.1 × 10 S/m and maintains stability after 10,000 stretch-release cycles at 40% strain. Compared with the conventional metal film electrode with a randomly wavy shape, the microconvex stripe-shaped platinum nanofilm significantly suppresses the strain concentration and the crack propagation of the nanofilm during the stretch-release cycles, resulting in the resistance after 1000 cycles being half that of conventional electrodes. The pressure sensor, based on the proposed electrode, has been shown to possess excellent fatigue resistance with only a 4% change in sensitivity after fatigue. The stretchable electrode based on a microconvex stripe-shaped platinum nanofilm on the elastomer provides an innovative solution for the long-term stable operation of stretchable electronics.
可拉伸电子器件面临长期稳定运行的挑战,其中一个困难在于核心部件电极在多次可拉伸变形下保持高导电性。为解决这一问题,我们提出一种高度抗疲劳的可拉伸金属薄膜电极,它由预弯曲成规则微凸条纹的铂纳米薄膜构成,位于弹性体材料表面。该可拉伸电极的电导率为4.1×10 S/m,在40%应变下经过10000次拉伸-释放循环后仍保持稳定。与具有随机波浪形状的传统金属薄膜电极相比,微凸条纹状铂纳米薄膜在拉伸-释放循环过程中显著抑制了纳米薄膜的应变集中和裂纹扩展,使得1000次循环后的电阻仅为传统电极的一半。基于所提出电极的压力传感器已被证明具有出色的抗疲劳性能,疲劳后灵敏度仅变化4%。基于弹性体上微凸条纹状铂纳米薄膜的可拉伸电极,为可拉伸电子器件的长期稳定运行提供了一种创新解决方案。