Panasiuk Mykola, Buzynnyi Mykhailo, Kirieiev Serhii, Sosonna Natalia, Kovalenko Ihor, Mykhailova Liubov
Institute for Safety Problems of Nuclear Power Plants, National Academy of Sciences of Ukraine, 36a Kirova Street, Chornobyl, 07270, Ukraine.
State Institution O.M. Marzieiev Institute of Public Health of National Academy of Medical Sciences of Ukraine, 50, Hetman Pavlo Polubotko Str, Kyiv, 02094, Ukraine.
Sci Rep. 2025 Apr 22;15(1):13910. doi: 10.1038/s41598-025-99095-5.
Wood contamination in the Chornobyl Exclusion Zone (CEZ) with Cs and Sr reaches tens of kBq/kg. Fires are natural disasters that fundamentally alter the forest ecosystem. The largest fires in the CEZ occurred in 2020 at the temporary radioactive waste storage facility (PTLRW) known as "Red Forest", where the peak of Sr activity in wood was recorded. Subsequently, the level of Sr in groundwater samples from observation wells in this section of the CEZ increased by 2 to 60 times, rising from approximately 2 to about 180 Bq/l beginning in late 2022. The laboratory experiment utilized typical pinewood and forest litter samples. Laboratory studies show that burning 1 kg of dry pinewood produces approximately 2.8 g of ash, with a concentration of 90Sr in the ash that is approximately 360 times higher. The specific activity of Sr in the ash from six wood samples ranged from 160 to 3400 kBq/kg. Under suitable experimental conditions, the specific activity of Sr in the leachate samples ranged from 0.5 to 0.72 kBq/L. The proportion of Sr leached during the experiment varied from 12 to 33% for wood ash and 10.8-13.2% for forest litter ash. The complete combustion of 10% of the wood in the burn site area of the PTLRW "Red Forest" CEZ, influenced by a two-year rainfall volume, releases a secondary source of 90Sr available for migration with groundwater, with an intensity of at least 0.69 GBq/ha or more than 17 GBq/ha in the trench burial area of "Red Forest". Under these conditions, this source can reach 38 TBq in the 550 km² burn site area. The minerals in wood ash are easily washed away by water, leading to increased groundwater mineralization and higher ionic strength. This, in turn, reduces the soil's sorption capacity and enhances the migration capacity of Sr in the aquifer. The transformation of wood and forest litter into ash due to a forest fire concentrates radioactivity in it, which lies on the soil surface, making it vulnerable to rapid leaching by atmospheric precipitation. As a result, this radioactivity can become a significant local source of radioactive contamination of surface and groundwater, which requires updating the radioactivity monitoring regulations in the relevant observation wells of the CEZ.
切尔诺贝利禁区(CEZ)内木材受铯和锶污染,含量达数十kBq/kg。火灾是从根本上改变森林生态系统的自然灾害。CEZ最大的火灾发生在2020年,地点是被称为“红色森林”的临时放射性废物储存设施(PTLRW),这里记录到木材中锶活度的峰值。随后,CEZ该区域观测井地下水样本中的锶含量从2022年末开始从约2 Bq/l增加到约180 Bq/l,增长了2至60倍。实验室实验使用了典型的松木和森林凋落物样本。实验室研究表明,燃烧1千克干燥松木产生约2.8克灰烬,灰烬中90Sr的浓度约高360倍。六个木材样本灰烬中锶的比活度范围为160至3400 kBq/kg。在合适的实验条件下,渗滤液样本中锶的比活度范围为0.5至0.72 kBq/L。实验期间,木材灰分中锶的淋溶比例为12%至33%,森林凋落物灰分为10.8%至13.2%。受两年降雨量影响,CEZ“红色森林”PTLRW燃烧场地10%的木材完全燃烧,释放出一个可供90Sr随地下水迁移的二次源,在“红色森林”的壕沟埋葬区强度至少为0.69 GBq/ha或超过17 GBq/ha。在这些条件下,这个源在550平方公里的燃烧场地面积内可达38 TBq。木材灰分中的矿物质很容易被水冲走,导致地下水矿化度增加和离子强度升高。这反过来又降低了土壤的吸附能力,增强了锶在含水层中的迁移能力。森林火灾导致木材和森林凋落物变成灰烬,使放射性集中在灰烬中,而灰烬位于土壤表面,容易被大气降水迅速淋溶。因此,这种放射性可能成为地表水和地下水放射性污染的一个重要局部来源,这就需要更新CEZ相关观测井的放射性监测规定。