Zhang Yanyu, Song Qianju, Hou Bin, Yi Zao
Opt Lett. 2025 May 1;50(9):2868-2871. doi: 10.1364/OL.558495.
Chiral metasurfaces supporting bound states in the continuum (BICs) have been extensively researched and gradually applied in biology, sensing, and optical communication due to their strong chiroptical response and ultrahigh-quality () factor. Here, we suggest a feasible pathway to realize steerable chiral metasurfaces with near-unity circular dichroism (CD), high figure of merit (FOM), and sensing sensitivity supported by a toroidal dipole (TD) response, that empower BICs. Through the study of symmetry of metasurfaces, we find that when the up-down and rotational symmetry of the system are broken, one circular () polarization state, carrying a fractional topological charge and separated from the eliminated BIC, can be moved to the Γ point, thereby forming a chiral quasi-BIC mode. The intrinsic chirality induced by the chiral quasi-BIC mode can be tuned over a wide frequency range and maintain a large CD value (>0.99) by virtue of the active tunable properties of bulk Dirac semimetal (BDS). We find that the chiral quasi-BIC mode is also dominated by TD through multipolar decomposition, which makes the mode possess high- factor. The chiral quasi-BIC mode can hold high FOM and sensing sensitivity (S) as the analyte changes. The proposed active tunable chiral metasurfaces can achieve excellent sensing characteristics in a variety of environments, which may have important applications in dynamic chiral detectors and other chiral optical instruments.
支持连续统束缚态(BICs)的手性超表面由于其强烈的手性光学响应和超高品质()因子,已得到广泛研究并逐渐应用于生物学、传感和光通信领域。在此,我们提出了一条可行的途径,以实现具有接近单位圆二色性(CD)、高优值(FOM)和由环形偶极子(TD)响应支持的传感灵敏度的可操纵手性超表面,该响应赋予了BICs特性。通过对超表面对称性的研究,我们发现当系统的上下对称性和旋转对称性被打破时,一个携带分数拓扑电荷且与消除的BIC分离的圆()偏振态可以移动到Γ点,从而形成一种手性准BIC模式。借助体狄拉克半金属(BDS)的主动可调特性,由手性准BIC模式诱导的固有手性可以在很宽的频率范围内进行调谐,并保持较大的CD值(>0.99)。我们发现,通过多极分解,手性准BIC模式也由TD主导,这使得该模式具有高品质因子。随着分析物的变化,手性准BIC模式可以保持较高的FOM和传感灵敏度(S)。所提出的主动可调手性超表面可以在各种环境中实现优异的传感特性,这可能在动态手性探测器和其他手性光学仪器中具有重要应用。