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环境物体中放射性碳的测定。

Determination of radiocarbon in environmental objects.

作者信息

Raimkanova Аlmira, Mamyrbayeva Ainur, Aidarkhanova Аlmira, Aidarkhanov Аssan, Sarsenova Aidana, Tleukanova Zhanna

机构信息

Institute of Radiation Safety and Ecology, National Nuclear Center of the Republic of Kazakhstan, Kurchatov, Kazakhstan.

出版信息

PLoS One. 2025 Jun 5;20(6):e0324818. doi: 10.1371/journal.pone.0324818. eCollection 2025.

DOI:10.1371/journal.pone.0324818
PMID:40471963
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC12140196/
Abstract

This article presents the results of radiocarbon distribution in natural components of 'Degelen' test location. It was used to conduct underground nuclear tests at the Semipalatinsk Test Site. Near-entry areas with water inflows were selected for research. Soil, plant and water samples were taken, in which the radiocarbon content was determined. The 14С activity concentration was determined using a highly sensitive alpha-beta radiometer SL-300 (ISO 13162, 2021). Sample preparation was carried out using a modern automated system Pyrolyser-6 Trio (Raddec International Ltd, UK). In the course of research undertaken, radiocarbon was revealed to be nonuniformly distributed in environmental objects. The effectiveness of Pyrolyser-6 Trio calcination and ashing system for 14C determination in environmental matrices has been demonstrated.

摘要

本文介绍了“杰格连”试验场自然组分中放射性碳分布的结果。该试验场曾用于在塞米巴拉金斯克试验场进行地下核试验。选择有水流流入的近入口区域进行研究。采集了土壤、植物和水样,并测定了其中的放射性碳含量。使用高灵敏度的α-β辐射计SL-300(ISO 13162,2021)测定了14С活度浓度。样品制备使用现代自动化系统Pyrolyser-6 Trio(英国Raddec International Ltd公司)进行。在研究过程中,发现放射性碳在环境物体中的分布不均匀。已证明Pyrolyser-6 Trio煅烧和灰化系统在环境基质中测定14C的有效性。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/fe15/12140196/642736cbb26f/pone.0324818.g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/fe15/12140196/80f22cdb0c8f/pone.0324818.g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/fe15/12140196/adf819a8d4ae/pone.0324818.g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/fe15/12140196/b1a1042ac9a9/pone.0324818.g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/fe15/12140196/642736cbb26f/pone.0324818.g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/fe15/12140196/80f22cdb0c8f/pone.0324818.g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/fe15/12140196/adf819a8d4ae/pone.0324818.g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/fe15/12140196/b1a1042ac9a9/pone.0324818.g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/fe15/12140196/642736cbb26f/pone.0324818.g004.jpg

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本文引用的文献

1
Assessment of the tritium distribution in the vegetation cover in the areas of underground nuclear explosions at the Semipalatinsk test site.评估塞米巴拉金斯克试验场地下核爆炸地区植被覆盖层中的氚分布。
J Environ Radioact. 2021 Oct;237:106705. doi: 10.1016/j.jenvrad.2021.106705. Epub 2021 Jul 27.
2
Optimisation of a batch thermal combustion method using a tube furnace oxidation system (pyrolyser) and LSC for carbon-14 determination in environmental matrices.优化使用管式炉氧化系统(热解器)和液体闪烁计数法进行环境基质中碳-14 测定的批量热燃烧法。
J Environ Radioact. 2021 Jan;226:106345. doi: 10.1016/j.jenvrad.2020.106345. Epub 2020 Oct 5.
3
Carbon-14 content in surface soils near atmospheric and below ground nuclear detonations.
地表土壤中碳-14 含量接近大气和地下核爆炸。
J Environ Radioact. 2019 Nov;208-209:106007. doi: 10.1016/j.jenvrad.2019.106007. Epub 2019 Jul 17.
4
Plants as indicators of tritium concentration in ground water at the Semipalatinsk test site.作为塞米巴拉金斯克试验场地下水氚浓度指示物的植物
J Environ Radioact. 2017 Oct;177:218-224. doi: 10.1016/j.jenvrad.2017.06.032. Epub 2017 Jul 13.
5
Nature of radioactive contamination of components of ecosystems of streamflows from tunnels of Degelen massif.杰格连地块隧道水流生态系统各组成部分的放射性污染性质。
J Environ Radioact. 2015 Jun;144:32-40. doi: 10.1016/j.jenvrad.2015.02.021. Epub 2015 Mar 17.
6
Comparison of radiocarbon techniques for the assessment of biobase content in fuels.用于评估燃料中生物基含量的放射性碳技术比较。
Appl Radiat Isot. 2014 Nov;93:106-9. doi: 10.1016/j.apradiso.2014.01.007. Epub 2014 Jan 30.
7
Tritium as an indicator of venues for nuclear tests.氚作为核试验场所的示踪剂。
J Environ Radioact. 2013 Oct;124:13-21. doi: 10.1016/j.jenvrad.2013.03.004. Epub 2013 Apr 29.
8
Effective desorption of tritium from diverse solid matrices and its application to routine analysis of decommissioning materials.有效解吸来自不同固体基质的氚及其在退役材料常规分析中的应用。
Anal Chim Acta. 2010 Aug 31;676(1-2):93-102. doi: 10.1016/j.aca.2010.07.017. Epub 2010 Jul 21.
9
(14)C, delta(13)C and total C content in soils around a Brazilian PWR nuclear power plant.巴西一座压水堆核电站周边土壤中的(14)C、δ(13)C和总碳含量。
J Environ Radioact. 2009 Apr;100(4):348-53. doi: 10.1016/j.jenvrad.2008.12.017. Epub 2009 Feb 11.
10
Carbon-14 in tree rings and other terrestrial samples in the vicinity of Ignalina Nuclear Power Plant, Lithuania.立陶宛伊格纳利纳核电站附近树木年轮及其他陆地样本中的碳-14。
J Environ Radioact. 2008 Feb;99(2):238-47. doi: 10.1016/j.jenvrad.2007.07.011. Epub 2007 Nov 13.