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生活污水是全球河流溶解碳中一个被忽视的来源和数量。

Domestic wastewater is an overlooked source and quantity in global river dissolved carbon.

作者信息

Cao Xingxing, Chen Shiqin, Liu Yan, Long Guangxi, Xu Y Jun

机构信息

College of Resources and Environmental Engineering, Guizhou University, Guiyang, China.

Key Laboratory of Karst Georesources and Environment (Guizhou University), Ministry of Education, Guiyang, China.

出版信息

Nat Commun. 2025 Aug 13;16(1):7522. doi: 10.1038/s41467-025-62920-6.

DOI:10.1038/s41467-025-62920-6
PMID:40804309
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC12350946/
Abstract

Riverine dissolved carbon (DC) plays a crucial role in global carbon cycle. Yet, the contribution of wastewater to global riverine DC remains unquantified. Here, we quantify the impact of treated and untreated domestic wastewater on dissolved inorganic carbon (DIC) and dissolved organic carbon (DOC) loadings at nation and river basin scales. We show that, globally, domestic wastewater discharges ~21.4 Tg DC annually-6.42 Tg DIC and 1.17 Tg DOC from treated, and 9.64 Tg DIC and 4.21 Tg DOC from untreated, collectively accounting for 3.13 ± 0.46% of the global riverine DC export. Contributions are highest in densely populated regions with high treatment capacity. Effluent DC levels are influenced by treatment technology, temperature, precipitation, economic growth and urban development. This underscores a need to incorporate the wastewater derived carbon into global carbon budget assessment, as well as to monitor and reduce carbon in wastewater effluents.

摘要

河流溶解碳(DC)在全球碳循环中起着至关重要的作用。然而,废水对全球河流DC的贡献仍未得到量化。在此,我们在国家和流域尺度上量化了经处理和未经处理的生活污水对溶解无机碳(DIC)和溶解有机碳(DOC)负荷的影响。我们表明,在全球范围内,生活污水每年排放约21.4 Tg DC——经处理的污水排放6.42 Tg DIC和1.17 Tg DOC,未经处理的污水排放9.64 Tg DIC和4.21 Tg DOC,合计占全球河流DC输出量的3.13±0.46%。在人口密集且处理能力高的地区,贡献最大。污水DC水平受处理技术、温度、降水、经济增长和城市发展的影响。这凸显了将废水中的碳纳入全球碳预算评估以及监测和减少废水排放中的碳的必要性。

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本文引用的文献

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Water Res. 2025 Jun 15;278:123415. doi: 10.1016/j.watres.2025.123415. Epub 2025 Feb 28.
2
Anthropogenic Water Withdrawals Modify Freshwater Inorganic Carbon Fluxes across the United States.人为取水改变了美国淡水无机碳通量。
Environ Sci Technol. 2025 Mar 4;59(8):3949-3960. doi: 10.1021/acs.est.4c09426. Epub 2025 Feb 17.
3
Wastewater-effluent discharge and incomplete denitrification drive riverine CO, CH and NO emissions.
废水排放和不完全反硝化作用导致河流中一氧化碳、甲烷和一氧化二氮的排放。
Sci Total Environ. 2024 Nov 15;951:175797. doi: 10.1016/j.scitotenv.2024.175797. Epub 2024 Aug 26.
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Land use and urbanization indirectly control riverine CH and CO emissions by altering nutrient input.土地利用和城市化通过改变养分输入间接控制河流 CH 和 CO 的排放。
Water Res. 2024 Nov 1;265:122266. doi: 10.1016/j.watres.2024.122266. Epub 2024 Aug 14.
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A critical review of characteristics of domestic wastewater and key treatment techniques in Chinese villages.中国农村生活污水特征及关键处理技术的综述评价
Sci Total Environ. 2024 Jun 1;927:172155. doi: 10.1016/j.scitotenv.2024.172155. Epub 2024 Apr 2.
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Connectivity of floodplain influences riverine carbon outgassing and dissolved carbon transport.洪泛平原的连通性影响河流碳的脱气和溶解碳的输送。
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