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通过核磁共振研究压力下18%硫取代的FeSe中源自博戈留波夫费米面的准粒子相互作用。

Quasiparticle interaction originating from Bogoliubov Fermi surfaces under pressure in 18%-S substituted FeSe studied via NMR.

作者信息

Yu Zhongyu, Shen Xiaoling, Nakamura Koya, Inomata Kazuya, Matsuura Kohei, Mizukami Yuta, Kasahara Shigeru, Matsuda Yuji, Shibauchi Takasada, Uwatoko Yoshiya, Fujiwara Naoki

机构信息

Graduate School of Human and Environmental Studies, Kyoto University, Yoshida-Nihonmatsu-cho, Sakyo-ku, Kyoto, 606-8501, Japan.

Institute for Solid State Physics, University of Tokyo, 5-1-5 Kashiwanoha, Kashiwa, 277-8581, Chiba, Japan.

出版信息

Sci Rep. 2025 Aug 14;15(1):29824. doi: 10.1038/s41598-025-13717-6.

Abstract

S-substituted FeSe superconductors in the tetragonal phase display several unique features among iron-based superconductors, particularly the presence of zero-energy excitations in the superconducting (SC) state. The recent concept of Bogoliubov Fermi surfaces (BFSs)-a theoretical model describing ultranodal states-has attracted considerable interest. Nuclear magnetic resonance (NMR) studies on FeSeS (x = 0.18) have revealed an anomalous low-energy spin fluctuations deep in the SC state. The low-energy spin fluctuations are enhanced with decreasing temperature, supporting strong Bogoliubov quasiparticle interactions associated with BFSs. Here, we further investigate these correlation effects through Se-NMR measurements of FeSeS (x = 0.18) under pressures up to 2.0 GPa and temperatures down to ~ 100 mK. The results demonstrate that the anomalous enhancement is suppressed but persists under pressure, implying that quasiparticle interactions become weak by applying pressure. Furthermore, spin fluctuations in the normal state exhibit different temperature dependence from those deep in the SC state, suggesting that the nesting properties of normal electrons differ from those of Bogoliubov quasiparticles. These findings are consistent with the theoretical model of BFSs with C symmetry and strengthen evidence for Bogoliubov quasiparticle interactions, providing insights into the unconventional pairing state of this system.

摘要

四方相的S取代FeSe超导体在铁基超导体中展现出几个独特的特征,特别是在超导(SC)态中存在零能激发。最近关于博戈留波夫费米面(BFSs)的概念——一种描述超节点态的理论模型——引起了相当大的关注。对FeSeS(x = 0.18)的核磁共振(NMR)研究揭示了在SC态深处存在反常的低能自旋涨落。低能自旋涨落随着温度降低而增强,这支持了与BFSs相关的强博戈留波夫准粒子相互作用。在此,我们通过在高达2.0 GPa的压力和低至约100 mK的温度下对FeSeS(x = 0.18)进行Se-NMR测量,进一步研究这些关联效应。结果表明,反常增强被抑制,但在压力下仍然存在,这意味着通过施加压力准粒子相互作用变弱。此外,正常态下的自旋涨落表现出与SC态深处不同的温度依赖性,这表明正常电子的嵌套性质与博戈留波夫准粒子的不同。这些发现与具有C对称性的BFSs理论模型一致,并加强了博戈留波夫准粒子相互作用的证据,为该系统的非常规配对态提供了见解。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e199/12354710/fecb0ca80761/41598_2025_13717_Fig1_HTML.jpg

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