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利用光子关联和量子照明领域的新兴方法提升光谱学和显微镜技术。

Enhancing spectroscopy and microscopy with emerging methods in photon correlation and quantum illumination.

作者信息

Tsao Chieh, Ling Haonan, Hinkle Alex, Chen Yifan, Jha Keshav Kumar, Yan Zhen-Li, Utzat Hendrik

机构信息

Department of Chemistry, University of California, Berkeley, Berkeley, CA, USA.

Materials Science Division, Lawrence Berkeley National Laboratory, Berkeley, CA, USA.

出版信息

Nat Nanotechnol. 2025 Aug 20. doi: 10.1038/s41565-025-01992-3.

DOI:10.1038/s41565-025-01992-3
PMID:40835979
Abstract

Quantum optics has led to important advancements in our ability to prepare and detect correlations between individual photons. Its principles are increasingly translated into nanoscale characterization tools, furthering methods in spectroscopy, microscopy and metrology. In this Review, we discuss the rapid progress in this field driven by advanced technologies of single-photon detectors and quantum-light sources, including time-resolved single-photon counting cameras, superconducting nanowire single-photon detectors and entangled photon sources of increasing brightness. We emphasize emerging applications in super-resolution microscopy, measurements below classical noise limits and photon-number-resolved spectroscopy-a powerful paradigm for the characterization of nanoscale electronic materials. We conclude by discussing key technological challenges and future opportunities in materials science and bionanophotonics alike.

摘要

量子光学在我们制备和探测单个光子之间相关性的能力方面取得了重要进展。其原理正越来越多地转化为纳米级表征工具,推动了光谱学、显微镜学和计量学方法的发展。在本综述中,我们讨论了由单光子探测器和量子光源等先进技术推动的该领域的快速进展,包括时间分辨单光子计数相机、超导纳米线单光子探测器以及亮度不断提高的纠缠光子源。我们强调了超分辨率显微镜、低于经典噪声极限的测量以及光子数分辨光谱学等新兴应用——这是一种用于表征纳米级电子材料的强大范例。我们通过讨论材料科学和生物纳米光子学中的关键技术挑战和未来机遇来结束本文。

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Tunable entangled photon-pair generation in a liquid crystal.液晶中可调谐的纠缠光子对的产生。
Nature. 2024 Jul;631(8020):294-299. doi: 10.1038/s41586-024-07543-5. Epub 2024 Jun 12.
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Quantum imaging of biological organisms through spatial and polarization entanglement.通过空间和偏振纠缠对生物有机体进行量子成像。
Sci Adv. 2024 Mar 8;10(10):eadk1495. doi: 10.1126/sciadv.adk1495.
4
Single-photon superradiance in individual caesium lead halide quantum dots.单个铯铅卤量子点中的单光子超辐射。
Nature. 2024 Feb;626(7999):535-541. doi: 10.1038/s41586-023-07001-8. Epub 2024 Jan 31.
5
A superconducting nanowire single-photon camera with 400,000 pixels.一种具有 40 万个像素的超导纳米线单光子相机。
Nature. 2023 Oct;622(7984):730-734. doi: 10.1038/s41586-023-06550-2. Epub 2023 Oct 25.
6
Fluorescence lifetime measurements using photon pair correlations generated via spontaneous parametric down conversion (SPDC).利用通过自发参量下转换(SPDC)产生的光子对关联进行荧光寿命测量。
Opt Express. 2023 Jul 31;31(16):26935-26947. doi: 10.1364/OE.494744.
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Time-Resolved Line Shapes of Single Quantum Emitters via Machine Learned Photon Correlations.通过机器学习光子相关性实现单量子发射器的时间分辨线形
Phys Rev Lett. 2023 Aug 4;131(5):053603. doi: 10.1103/PhysRevLett.131.053603.
8
Machine learning assisted quantum super-resolution microscopy.机器学习辅助量子超分辨率显微镜。
Nat Commun. 2023 Aug 10;14(1):4828. doi: 10.1038/s41467-023-40506-4.
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Two Biexciton Types Coexisting in Coupled Quantum Dot Molecules.耦合量子点分子中共存的两种双激子类型。
ACS Nano. 2023 Aug 8;17(15):14990-15000. doi: 10.1021/acsnano.3c03921. Epub 2023 Jul 17.
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Entangled Photon Correlations Allow a Continuous-Wave Laser Diode to Measure Single-Photon, Time-Resolved Fluorescence.纠缠光子相关使得连续波激光二极管能够测量单光子、时间分辨荧光。
J Phys Chem Lett. 2023 Jun 29;14(25):5805-5811. doi: 10.1021/acs.jpclett.3c01266. Epub 2023 Jun 20.