铁硫蛋白活性位点的合成类似物。II. 四（巯基 - μ³ - 硫代 - 铁）簇合物(Fe₄S₄(SR)₄)²⁻的合成与结构 - Suppr

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Synthetic analogs of the active sites of iron-sulfur proteins. II. Synthesis and structure of the tetra(mercapto-m 3 -sulfido-iron) clusters, (Fe 4 S 4 (SR) 4 ) 2- .

作者信息

Averill B A, Herskovitz T, Holm R H, Ibers J A

出版信息

J Am Chem Soc. 1973 May 30;95(11):3523-34. doi: 10.1021/ja00792a013.

DOI:10.1021/ja00792a013

PMID:4708377

Abstract

摘要

相似文献

Synthetic analogs of the active sites of iron-sulfur proteins. II. Synthesis and structure of the tetra(mercapto-m 3 -sulfido-iron) clusters, (Fe 4 S 4 (SR) 4 ) 2- .

J Am Chem Soc. 1973 May 30;95(11):3523-34. doi: 10.1021/ja00792a013.

Synthetic analogs of the active sites of iron-sulfur proteins; X. Kinetics and mechanism of the ligand substitution reactions of arylthiols with the tetranuclear clusters [Fe4S4(SR)4]2 minus;

J Am Chem Soc. 1975 Feb 5;97(3):528-33. doi: 10.1021/ja00836a011.

Synthetic analogs of the active sites of iron-sulfur proteins. VII. Ligand substitution reactions of the tetranuclear clusters (Fe4S4(SR)4)2- and the structure of ((CH3)4N)2(Fe4S4(SC6H5)4).

J Am Chem Soc. 1974 Jun 26;96(13):4168-78. doi: 10.1021/ja00820a018.

Synthetic analogs of the active sites of iron-sulfur proteins. V. Proton resonance properties of the tetranuclear clusters (Fe4S4(SR)4). Evidence for dominant contact interactions.

J Am Chem Soc. 1974 Apr 3;96(7):2109-17. doi: 10.1021/ja00814a020.

Synthetic analogs of the active sites of iron-sulfur proteins. 8. Some electronic properties of (Fe4S4(SR)4)3-, analogs of reduced bacterial ferredoxins.

Biochem Biophys Res Commun. 1974 Jun 18;58(4):974-82. doi: 10.1016/s0006-291x(74)80239-1.

Synthesis and reactions of cubane-type iron-sulfur-phosphine clusters, including soluble clusters of nuclearities 8 and 16.

Inorg Chem. 2003 Jan 13;42(1):11-21. doi: 10.1021/ic020464t.

Tridentate thiolate ligands: application to the synthesis of the site-differentiated [4Fe-4S] cluster having a hydrosulfide ligand at the unique iron center.

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Synthetic analogs of the active sites of iron-sulfur proteins. VI. Spectral and redox characteristics of the tetranuclear clusters (Fe4S4(SR)4).2-.

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Synthetic analogs of active sites of iron-sulfur proteins: bis (o-xylyldithiolato) ferrate (III) monoanion, a structurally unconstrained model for the rubredoxin Fe-S4 unit.

Proc Natl Acad Sci U S A. 1975 Aug;72(8):2868-72. doi: 10.1073/pnas.72.8.2868.

Synthetic analogs of the active sites of iron-sulfur proteins. IV. Ligand substitution reactions of the tetranuclear clusters (Fe4S4(SR)4)2-.

J Am Chem Soc. 1974 Jan 9;96(1):285-7. doi: 10.1021/ja00808a064.

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Synthetic analogs of the active sites of iron-sulfur proteins. II. Synthesis and structure of the tetra(mercapto-m 3 -sulfido-iron) clusters, (Fe 4 S 4 (SR) 4 ) 2- .

作者信息

Averill B A, Herskovitz T, Holm R H, Ibers J A

出版信息

J Am Chem Soc. 1973 May 30;95(11):3523-34. doi: 10.1021/ja00792a013.

DOI:10.1021/ja00792a013

PMID:4708377

Abstract

摘要

相似文献

Synthetic analogs of the active sites of iron-sulfur proteins. II. Synthesis and structure of the tetra(mercapto-m 3 -sulfido-iron) clusters, (Fe 4 S 4 (SR) 4 ) 2- .

J Am Chem Soc. 1973 May 30;95(11):3523-34. doi: 10.1021/ja00792a013.

Synthetic analogs of the active sites of iron-sulfur proteins; X. Kinetics and mechanism of the ligand substitution reactions of arylthiols with the tetranuclear clusters [Fe4S4(SR)4]2 minus;

J Am Chem Soc. 1975 Feb 5;97(3):528-33. doi: 10.1021/ja00836a011.

Synthetic analogs of the active sites of iron-sulfur proteins. VII. Ligand substitution reactions of the tetranuclear clusters (Fe4S4(SR)4)2- and the structure of ((CH3)4N)2(Fe4S4(SC6H5)4).

J Am Chem Soc. 1974 Jun 26;96(13):4168-78. doi: 10.1021/ja00820a018.

Synthetic analogs of the active sites of iron-sulfur proteins. V. Proton resonance properties of the tetranuclear clusters (Fe4S4(SR)4). Evidence for dominant contact interactions.

J Am Chem Soc. 1974 Apr 3;96(7):2109-17. doi: 10.1021/ja00814a020.

Synthetic analogs of the active sites of iron-sulfur proteins. 8. Some electronic properties of (Fe4S4(SR)4)3-, analogs of reduced bacterial ferredoxins.

Biochem Biophys Res Commun. 1974 Jun 18;58(4):974-82. doi: 10.1016/s0006-291x(74)80239-1.

Synthesis and reactions of cubane-type iron-sulfur-phosphine clusters, including soluble clusters of nuclearities 8 and 16.

Inorg Chem. 2003 Jan 13;42(1):11-21. doi: 10.1021/ic020464t.

Tridentate thiolate ligands: application to the synthesis of the site-differentiated [4Fe-4S] cluster having a hydrosulfide ligand at the unique iron center.

Chem Asian J. 2012 May;7(5):920-9. doi: 10.1002/asia.201200039. Epub 2012 Apr 5.

Synthetic analogs of the active sites of iron-sulfur proteins. VI. Spectral and redox characteristics of the tetranuclear clusters (Fe4S4(SR)4).2-.

J Am Chem Soc. 1974 Jun 26;96(13):4159-67. doi: 10.1021/ja00820a017.

Synthetic analogs of active sites of iron-sulfur proteins: bis (o-xylyldithiolato) ferrate (III) monoanion, a structurally unconstrained model for the rubredoxin Fe-S4 unit.

Proc Natl Acad Sci U S A. 1975 Aug;72(8):2868-72. doi: 10.1073/pnas.72.8.2868.

Synthetic analogs of the active sites of iron-sulfur proteins. IV. Ligand substitution reactions of the tetranuclear clusters (Fe4S4(SR)4)2-.

J Am Chem Soc. 1974 Jan 9;96(1):285-7. doi: 10.1021/ja00808a064.

引用本文的文献

The Properties That Allow Tuning the Reduction Potentials over a Volt Range in Biological Iron/Sulfur Clusters.

J Phys Chem Lett. 2025 May 15;16(19):4602-4606. doi: 10.1021/acs.jpclett.5c00616. Epub 2025 May 1.

Understanding the P-Cluster of Vanadium Nitrogenase: an EPR and XAS Study of the Holo vs. Apo Forms of the Enzyme.

Chembiochem. 2025 Feb 1;26(3):e202400833. doi: 10.1002/cbic.202400833. Epub 2024 Dec 2.

Facile and dynamic cleavage of every iron-sulfide bond in cuboidal iron-sulfur clusters.

Proc Natl Acad Sci U S A. 2023 Feb 7;120(6):e2210528120. doi: 10.1073/pnas.2210528120. Epub 2023 Jan 31.

A complete biomimetic iron-sulfur cubane redox series.

Proc Natl Acad Sci U S A. 2022 Aug 2;119(31):e2122677119. doi: 10.1073/pnas.2122677119. Epub 2022 Jul 26.

Radical SAM-dependent formation of a nitrogenase cofactor core on NifB.

J Inorg Biochem. 2022 Aug;233:111837. doi: 10.1016/j.jinorgbio.2022.111837. Epub 2022 Apr 20.

Spin-Pure Stochastic-CASSCF via GUGA-FCIQMC Applied to Iron-Sulfur Clusters.

J Chem Theory Comput. 2021 Sep 14;17(9):5684-5703. doi: 10.1021/acs.jctc.1c00589. Epub 2021 Sep 1.

Phosphorus Kβ X-ray emission spectroscopy detects non-covalent interactions of phosphate biomolecules .

Chem Sci. 2021 Apr 29;12(22):7888-7901. doi: 10.1039/d1sc01266e.

Resolution of Low-Energy States in Spin-Exchange Transition-Metal Clusters: Case Study of Singlet States in [Fe(III)S] Cubanes.

J Phys Chem A. 2021 Jun 10;125(22):4727-4740. doi: 10.1021/acs.jpca.1c00397. Epub 2021 May 28.

Cleavage of cluster iron-sulfide bonds in cyclophane-coordinated FeS complexes.

Dalton Trans. 2021 Jan 21;50(3):816-821. doi: 10.1039/d0dt03805a. Epub 2021 Jan 4.

Tracing the 'ninth sulfur' of the nitrogenase cofactor via a semi-synthetic approach.

Nat Chem. 2018 May;10(5):568-572. doi: 10.1038/s41557-018-0029-4. Epub 2018 Apr 16.