Winterbourn C C, Carrell R W
J Clin Invest. 1974 Sep;54(3):678-89. doi: 10.1172/JCI107806.
The sequential changes that occur during the precipitation on mild heating of the unstable hemoglobins, Hb Christchurch, Hb Sydney, Hb Köln, and Hb A, were examined with particular attention to the possibility of an accompanying oxidative process. Hb Christchurch, Hb Sydney, and Hb A precipitated with equal amounts of alpha- and beta-chains and full heme complement. Hb Köln, however, was one-half hemedepleted and showed a slight excess of precipitated beta-chains. In all cases the spectrum of the precipitated material was typical of a hemichrome. There was no evidence that sulfhydryl oxidation contributed to the precipitation process. Reduced glutathione was unable to protect the hemoglobin against precipitation, and mixed disulfide formation between the precipitating hemoglobin and glutathione was insignificant, even in the presence of excess glutathione. No blockade of beta93 cysteines could be demonstrated in the unstable hemoglobins. Precipitation of oxyhemoglobin and carboxyhemoglobin in all cases gave nonspecific oxidation of approximately two of the six hemoglobin sulfhydryl groups to give intra- and intermolecular disulfide bonds. Single alpha- and beta-chains, plus polymers of up to five or six chains linked by disulfide bridges, were demonstrated by polyacrylamide gel electrophoresis. This disulfide oxidation was not observed with deoxy- or methemoglobin and did not appear to influence the rate of precipitation. These findings fit the theoretical prediction that autoxidation of oxy- and carboxyhemoglobin is accompanied by formation of a free radical, with the reactions of this free radical being confined intramolecularly.Together, these results are in keeping with predictions based on the known structural abnormalities of the unstable hemoglobins, all of which result in greater molecular flexibility. Our findings support the conclusion that the usual precipitating event is altered bonding at the heme to give the formation of hemichromes. There is no evidence of an accompanying oxidative process that could pose a threat to the integrity of the red cell.
研究了不稳定血红蛋白Hb Christchurch、Hb Sydney、Hb Köln和Hb A在温和加热沉淀过程中发生的一系列变化,特别关注了伴随氧化过程的可能性。Hb Christchurch、Hb Sydney和Hb A沉淀时α链和β链数量相等且血红素完整。然而,Hb Köln有一半血红素缺失,且沉淀的β链略有过量。在所有情况下,沉淀物质的光谱都是半色素的典型光谱。没有证据表明巯基氧化参与了沉淀过程。还原型谷胱甘肽无法保护血红蛋白免于沉淀,即使在存在过量谷胱甘肽的情况下,沉淀的血红蛋白与谷胱甘肽之间形成的混合二硫键也微不足道。在不稳定血红蛋白中未发现β93半胱氨酸被阻断。在所有情况下,氧合血红蛋白和羧基血红蛋白的沉淀都会使六个血红蛋白巯基中的大约两个发生非特异性氧化,形成分子内和分子间二硫键。通过聚丙烯酰胺凝胶电泳证明了单条α链和β链,以及由二硫键连接的多达五或六条链的聚合物。在脱氧血红蛋白或高铁血红蛋白中未观察到这种二硫键氧化,且它似乎不影响沉淀速率。这些发现符合理论预测,即氧合血红蛋白和羧基血红蛋白的自氧化伴随着自由基的形成,且该自由基的反应局限于分子内。总之,这些结果与基于不稳定血红蛋白已知结构异常的预测一致,所有这些异常都导致分子柔韧性增强。我们的发现支持这样的结论,即通常的沉淀事件是血红素处的键合改变,导致半色素的形成。没有证据表明伴随的氧化过程会对红细胞的完整性构成威胁。