Zaider M, Brenner D J
Radiat Res. 1984 Nov;100(2):245-56.
A Monte Carlo code was developed to stimulate stochastically the fast reactions of radiolysis products in water. The results of these calculations show that treatments based on deterministic kinetic rate equations do not reproduce correctly the evolution in time of the number of species. Ad hoc initial distributions of species in spurs, of the type used in deterministic approaches, are compared with more realistic distributions obtained from Monte Carlo-generated particle tracks. The effects of using either type of distribution, stochastically or deterministically, are discussed.
开发了一个蒙特卡罗代码，用于随机模拟水中辐射分解产物的快速反应。这些计算结果表明，基于确定性动力学速率方程的处理方法不能正确再现物种数量随时间的演变。将确定性方法中使用的那种类型的原初径迹中物种的临时初始分布，与从蒙特卡罗生成的粒子径迹获得的更现实的分布进行了比较。讨论了随机或确定性地使用这两种分布类型的影响。
