Fetisova Z G, Fok M V
Mol Biol (Mosk). 1984 Nov-Dec;18(6):1651-6.
It is shown, that the photosynthetic unit structure is to be strongly optimized in vivo to operate with a 90% quantum yield of primary charge separation in reaction centers, which means that a macroscopic photosynthetic unit is neither uniform nor isotropic. Some requirements for optimization of photosynthetic unit structure are determined. The modified probability matrix method to simulate the excitation energy transfer in photosynthesis is proposed. The method is adapted to excitation trapping time (but not to excitation jumps number) calculation. The calculations assume a Förster inductive resonance mechanism for energy transfer within light-harvesting antenna and pairwise dipolar interactions.
结果表明，光合作用单位结构在体内需要进行强烈优化，以便在反应中心以90%的初级电荷分离量子产率运行，这意味着宏观光合作用单位既不均匀也不是各向同性的。确定了光合作用单位结构优化的一些要求。提出了用于模拟光合作用中激发能量转移的修正概率矩阵方法。该方法适用于激发俘获时间（但不适用于激发跳跃次数）的计算。计算假设在光捕获天线内能量转移采用福斯特感应共振机制以及成对偶极相互作用。
