Müller-Newen G, Janssen U, Stoffel W
Institute of Biochemistry, Medical Faculty, University of Cologne, Germany.
Eur J Biochem. 1995 Feb 15;228(1):68-73. doi: 10.1111/j.1432-1033.1995.tb20230.x.
Mitochondrial 2-enoyl-CoA hydratase (mECH) and 3,2-trans-enoyl-CoA isomerase (mECI), two enzymes which catalyze totally different reactions in fatty acid beta-oxidation, belong to the low-similarity hydratase/isomerase enzyme superfamily. Their substrates and reaction mechanisms are similar [Müller-Newen, G. & Stoffel, W. (1993) Biochemistry 32, 11,405-11,412]. Glu164 of mECH is the only amino acid with a protic side chain that is conserved in these monofunctional and polyfunctional enzymes with 2-enoyl-CoA hydratase and 3,2-trans-enoyl-CoA isomerase activities. We tested our hypothesis that Glu164 of mECH is the putative active-site amino acid responsible for the base-catalyzed alpha-deprotonation in the hydratase/dehydrase and isomerase reaction. We functionally expressed rat liver mECH wild-type and [E164Q] mutant enzymes in Escherichia coli. Characterization of the purified wild-type and mutant enzymes revealed that the replacement of Glu164 by Gln lowers the kcat value more than 100,000-fold, whereas the Km value is only moderately affected. We have demonstrated in a previous study that Glu165 is indispensable for the 3,2-trans-enoyl-CoA isomerase activity. Taking these results together, we conclude that the conserved glutamic acid is the essential basic group in the active sites of 2-enoyl-CoA hydratase (Glu164) and 3,2-trans-enoyl-CoA isomerase (Glu165), and that these enzymes are not only evolutionarily but also functionally and mechanistically related.
线粒体2-烯酰辅酶A水合酶(mECH)和3,2-反式烯酰辅酶A异构酶(mECI)是两种在脂肪酸β-氧化中催化完全不同反应的酶,它们属于低相似性水合酶/异构酶超家族。它们的底物和反应机制相似[Müller-Newen, G. & Stoffel, W. (1993) Biochemistry 32, 11,405 - 11,412]。mECH的Glu164是唯一具有质子化侧链的氨基酸,在这些具有2-烯酰辅酶A水合酶和3,2-反式烯酰辅酶A异构酶活性的单功能和多功能酶中保守。我们测试了我们的假设,即mECH的Glu164是负责水合酶/脱水酶和异构酶反应中碱催化α-去质子化的假定活性位点氨基酸。我们在大肠杆菌中功能性表达了大鼠肝脏mECH野生型和[E164Q]突变酶。对纯化的野生型和突变酶的表征表明,用Gln取代Glu164使kcat值降低了100,000倍以上,而Km值仅受到适度影响。我们在先前的研究中已经证明Glu165对于3,2-反式烯酰辅酶A异构酶活性是不可或缺的。综合这些结果,我们得出结论,保守的谷氨酸是2-烯酰辅酶A水合酶(Glu164)和3,2-反式烯酰辅酶A异构酶(Glu165)活性位点中的必需碱性基团,并且这些酶不仅在进化上,而且在功能和机制上都是相关的。