Sorensen CM, Roberts GC
Department of Physics, Kansas State University, Manhattan, Kansas, 66506
J Colloid Interface Sci. 1997 Feb 15;186(2):447-52. doi: 10.1006/jcis.1996.4664.
The prefactor k0 of the fractal aggregate scaling relationship N = k0(Rg/a)Df is determined for both Diffusion Limited and Diffusion Limited Cluster Aggregation processes in spatial dimensions of 2, 3, 4, and 5. For the physically relevant case of DLCA aggregates in three dimensions we find k0 = 1.19 ± 0.1 when Df = 1.82 ± 0.04. Comparison of all aggregation types shows that the prefactor k0 displays uniform trends with the fractal dimension Df. Attempts to explain these trends are made based on either a common small N limit for all clusters or the packing of spheres in space.
分形聚集体标度关系N = k0(Rg/a)Df 的前置因子k0是针对二维、三维、四维和五维空间中的扩散受限和扩散受限簇聚过程确定的。对于三维空间中DLCA聚集体的实际相关情况,当Df = 1.82 ± 0.04时,我们发现k0 = 1.19 ± 0.1。对所有聚集类型的比较表明,前置因子k0与分形维数Df呈现出一致的趋势。基于所有簇的共同小N极限或空间中球体的堆积来尝试解释这些趋势。