Hurt J D, Tu C, Laipis P J, Silverman D N
Department of Biochemistry and Molecular Biology, University of Florida College of Medicine, Gainesville, Florida 32610-0267, USA.
J Biol Chem. 1997 May 23;272(21):13512-8. doi: 10.1074/jbc.272.21.13512.
A cDNA encoding the murine carbonic anhydrase IV (mCA IV) gene, modified to resemble a form of mature human carbonic anhydrase IV (Okuyama, T., Waheed, A., Kusumoto, W., Zhu, X. L., and Sly, W. S. (1995) Arch. Biochem. Biophys. 320, 315-322), was expressed in Escherichia coli. Inactive inclusion bodies were collected and refolded, and active enzyme was purified; the resulting mCA IV was used to characterize the catalysis of CO2 hydration using stopped flow spectrophotometry and 18O exchange between CO2 and water. Unlike previously studied isozymes in this class of carbonic anhydrase, the pH profile for kcat for hydration of CO2 catalyzed by mCA IV could not be described by a single ionization, suggesting multiple proton transfer pathways between the zinc-bound water molecule and solution. A role for His64 in transferring protons between the zinc-bound water and solution was confirmed by the 100-fold lower activity of the mutant of mCA IV containing the replacement His64 --> Ala. The remaining activity in this mutant at pH levels near 9 suggested a second proton shuttle mechanism. The maximal turnover number kcat for hydration of CO2 catalyzed by mCA IV was 1.1 x 10(6) s-1 at pH > 9. A pKa of 6.6 was estimated for the zinc-bound water molecule in mCA IV.
编码鼠碳酸酐酶IV(mCA IV)基因的cDNA经过修饰,使其类似于成熟的人碳酸酐酶IV的形式(冈山县,T.,瓦希德,A.,久留本,W.,朱,X.L.,和斯利,W.S.(1995年)《生物化学与生物物理学报》320,315 - 322),在大肠杆菌中表达。收集无活性的包涵体并进行复性,然后纯化活性酶;所得的mCA IV用于通过停流分光光度法和CO₂与水之间的¹⁸O交换来表征CO₂水合的催化作用。与此前研究的这类碳酸酐酶中的同工酶不同,mCA IV催化CO₂水合反应的kcat的pH曲线不能用单一的电离来描述,这表明在锌结合的水分子与溶液之间存在多条质子转移途径。通过将His64替换为Ala的mCA IV突变体活性降低100倍,证实了His64在锌结合水与溶液之间转移质子的作用。该突变体在pH接近9时的剩余活性表明存在第二种质子穿梭机制。在pH > 9时,mCA IV催化CO₂水合反应的最大周转数kcat为1.1×10⁶ s⁻¹。估计mCA IV中锌结合水分子的pKa为6.6。