Rønnow H M, McMorrow D F, Coldea R, Harrison A, Youngson I D, Perring T G, Aeppli G, Syljuåsen O, Lefmann K, Rischel C
Condensed Matter Physics and Chemistry Department, Risø National Laboratory, DK-4000 Roskilde, Denmark.
Phys Rev Lett. 2001 Jul 16;87(3):037202. doi: 10.1103/PhysRevLett.87.037202. Epub 2001 Jun 28.
The magnetic excitation spectrum in the two-dimensional (2D) S = 1/2 Heisenberg antiferromagnet copper deuteroformate tetradeuterate has been measured for temperatures up to T approximately J/2, where J = 6.31+/-0.02 meV is the 2D exchange coupling. For T<<J, a dispersion of the zone boundary energy is observed, which is attributed to a wave vector dependent quantum renormalization. At higher temperatures, spin-wavelike excitations persist, but are found to broaden and soften. By combining our data with numerical calculations, and with existing theoretical work, a consistent description of the behavior of the model system is found over the whole temperature interval investigated.