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自旋1/2三角晶格海森堡反铁磁体BaCoSbO中磁激发的结构

Structure of the magnetic excitations in the spin-1/2 triangular-lattice Heisenberg antiferromagnet BaCoSbO.

作者信息

Ito Saya, Kurita Nobuyuki, Tanaka Hidekazu, Ohira-Kawamura Seiko, Nakajima Kenji, Itoh Shinichi, Kuwahara Keitaro, Kakurai Kazuhisa

机构信息

Department of Physics, Tokyo Institute of Technology, Oh-okayama, Meguro-ku, Tokyo, 152-8551, Japan.

Materials and Life Science Division, J-PARC Center, Tokai, Ibaraki, 319-1195, Japan.

出版信息

Nat Commun. 2017 Aug 10;8(1):235. doi: 10.1038/s41467-017-00316-x.

Abstract

A spin-1/2 triangular-lattice Heisenberg antiferromagnet (TLHAF) is a prototypical frustrated quantum magnet, which exhibits remarkable quantum many-body effects that arise from the synergy between spin frustration and quantum fluctuation. The ground-state properties of a spin-1/2 TLHAF are theoretically well understood. However, the theoretical consensus regarding the magnetic excitations is limited. The experimental study of the magnetic excitations in spin-1/2 TLHAFs has also been limited. Here we show the structure of magnetic excitations in the spin-1/2 TLHAF BaCoSbO investigated by inelastic neutron scattering. Significantly different from theoretical expectations, the excitation spectrum has a three-stage energy structure. The lowest-energy first stage is composed of dispersion branches of single-magnon excitations. The second and third stages are dispersive continua accompanied by a columnar continuum extending above 10 meV, which is six times larger than the exchange interaction J = 1.67 meV. Our results indicate the shortcomings of the current theoretical framework.Two-dimensional frustrated magnets are heavily studied because theories predict that quantum effects may lead to the emergence of fractionalized excitations. Ito et al. use inelastic neutron scattering to show that the excitation spectrum of BaCoSbO disagrees with current theoretical expectations.

摘要

自旋为1/2的三角晶格海森堡反铁磁体(TLHAF)是一种典型的受挫量子磁体,它展现出由自旋受挫和量子涨落之间的协同作用产生的显著量子多体效应。自旋为1/2的TLHAF的基态性质在理论上已得到很好的理解。然而,关于磁激发的理论共识有限。对自旋为1/2的TLHAF中的磁激发的实验研究也很有限。在此,我们展示了通过非弹性中子散射研究的自旋为1/2的TLHAF BaCoSbO中的磁激发结构。与理论预期显著不同的是,激发谱具有三阶段能量结构。能量最低的第一阶段由单磁振子激发的色散分支组成。第二和第三阶段是色散连续区,伴有一个延伸至10 meV以上的柱状连续区,这比交换相互作用J = 1.67 meV大六倍。我们的结果表明了当前理论框架的不足之处。二维受挫磁体受到大量研究,因为理论预测量子效应可能导致分数化激发的出现。伊藤等人利用非弹性中子散射表明,BaCoSbO的激发谱与当前理论预期不一致。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/d7ef/5550445/94a4dfbf3156/41467_2017_316_Fig1_HTML.jpg

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