Stoycheva Antitsa D, Singer Sherwin J
Department of Chemistry, Ohio State University, 100 W. 18th Avenue, Columbus, Ohio 43210, USA.
Phys Rev E Stat Nonlin Soft Matter Phys. 2002 Mar;65(3 Pt 2B):036706. doi: 10.1103/PhysRevE.65.036706. Epub 2002 Feb 19.
The results and methodology of large scale computer simulations of the two-dimensional dipolar Ising model with long-range interactions are reported. Systems as large as 117,649 particles were studied to elucidate the elementary excitations and phase diagram of two-dimensional systems, such as Langmuir monolayers, thin garnet films, and adsorbed films on solid surfaces, which spontaneously form patterns of stripes, bubbles, and intermediately shaped domains. The challenging numerical investigations of large scale systems with long-range interactions at low temperatures were made possible by combining the fast multipole method and a non-Metropolis Monte Carlo sampling technique. Our simulations provide evidence that, at sufficiently high ratios of the repulsive to the attractive coupling constant for the model, twofold stripe order in the systems of interest is lost through a defect-mediated mechanism. Heat capacity data and the excitations observed in our simulations as the system disorders indicate that it is most likely an instance of a Kosterlitz-Thouless phase transition. The results from simulations with and without external field are in excellent agreement with the predictions of an analytic scaling theory [A. D. Stoycheva and S. J. Singer, Phys. Rev. E 64, 016118 (2001)], confirming the phase diagram furnished by the analytic model. The scaling theory suggests that, under certain conditions, defect-mediated stripe melting may be supplanted by Ising like disordering within stripes for small repulsion strength. A qualitative discussion of a model that supports both disordering mechanisms is presented.
报道了具有长程相互作用的二维偶极伊辛模型的大规模计算机模拟结果和方法。研究了多达117,649个粒子的系统,以阐明二维系统的基本激发和相图,如朗缪尔单层、石榴石薄膜以及固体表面的吸附膜,这些系统会自发形成条纹、气泡和中间形状的畴图案。通过结合快速多极方法和非梅特罗波利斯蒙特卡罗采样技术,实现了对低温下具有长程相互作用的大规模系统的具有挑战性的数值研究。我们的模拟提供了证据,即在该模型中,当排斥耦合常数与吸引耦合常数的比值足够高时,相关系统中的双重条纹序会通过缺陷介导机制消失。我们模拟中系统无序时观测到的热容量数据和激发表明,这很可能是一个Kosterlitz-Thouless相变的实例。有无外场情况下的模拟结果与解析标度理论[A. D. Stoycheva和S. J. Singer, Phys. Rev. E 64, 016118 (2001)]的预测非常吻合,证实了解析模型给出的相图。标度理论表明,在某些条件下,对于小的排斥强度,缺陷介导的条纹熔化可能会被条纹内类似伊辛的无序所取代。本文给出了一个支持两种无序机制的模型的定性讨论。