Yiou F, Raisbeck G M, Christensen G C, Holm E
Centre de Spectrométrie Nucléaire et de Spectrométrie de Masse, IN2P3-CNRS, Orsay, France.
J Environ Radioact. 2002;60(1-2):61-71. doi: 10.1016/s0265-931x(01)00096-0.
Discharges of the nuclides 129I, 137Cs and 99Tc from the nuclear reprocessing facilities at Sellafield (UK) and La Hague (France) are very useful as oceanic tracers. On the basis of 129I/127I, 137Cs and 99Tc measurements in archived seaweeds, the ratios of 129I/127I, 129I/137Cs and 129I/99Tc have been estimated in seawater at two locations (Utsira and Kiberg) in the Norwegian Coastal Current from 1980 to 1998. These ratios, which vary up to two orders of magnitude over this period, are potentially very interesting for determining "transit times" in the Arctic and North Atlantic oceans. While the long-term trends in these ratios are quite clear, measurements in monthly and bimonthly samples show considerable structure. Further studies are required to determine the exact origin of this structure, which may be a limiting factor in the time resolution that can be obtained with these parameters.
英国塞拉菲尔德和法国拉阿格的核后处理设施排放的核素129I、137Cs和99Tc作为海洋示踪剂非常有用。基于对存档海藻中129I/127I、137Cs和99Tc的测量,已估算出1980年至1998年挪威沿岸流中两个地点(乌茨拉和基伯格)海水中的129I/127I、129I/137Cs和129I/99Tc比值。在此期间,这些比值变化高达两个数量级,对于确定北冰洋和北大西洋的“过境时间”可能非常有趣。虽然这些比值的长期趋势相当明显,但月度和双月样本的测量显示出相当大的结构。需要进一步研究来确定这种结构的确切来源,这可能是这些参数所能获得的时间分辨率的一个限制因素。