Hwang J, Timusk T, Gu G D
Department of Physics and Astronomy, McMaster University, Hamilton, Ontario L8S 4M1, Canada.
Nature. 2004 Feb 19;427(6976):714-7. doi: 10.1038/nature02347.
The fundamental mechanism that gives rise to high-transition-temperature (high-T(c)) superconductivity in the copper oxide materials has been debated since the discovery of the phenomenon. Recent work has focused on a sharp 'kink' in the kinetic energy spectra of the electrons as a possible signature of the force that creates the superconducting state. The kink has been related to a magnetic resonance and also to phonons. Here we report that infrared spectra of Bi2Sr2CaCu2O8+delta (Bi-2212), shows that this sharp feature can be separated from a broad background and, interestingly, weakens with doping before disappearing completely at a critical doping level of 0.23 holes per copper atom. Superconductivity is still strong in terms of the transition temperature at this doping (T(c) approximately 55 K), so our results rule out both the magnetic resonance peak and phonons as the principal cause of high-T(c) superconductivity. The broad background, on the other hand, is a universal property of the copper-oxygen plane and provides a good candidate signature of the 'glue' that binds the electrons.
自铜氧化物材料中发现高温超导现象以来,其产生高温转变温度(高Tc)超导性的基本机制一直存在争议。最近的研究工作聚焦于电子动能谱中的一个尖锐“扭结”,将其作为产生超导态的力的一种可能特征。该扭结与磁共振以及声子都有关联。在此,我们报告Bi2Sr2CaCu2O8+δ(Bi-2212)的红外光谱表明,这一尖锐特征能够从一个宽泛的背景中分离出来,有趣的是,它在掺杂过程中会减弱,直至在每个铜原子0.23个空穴的临界掺杂水平时完全消失。在这个掺杂水平下,就转变温度而言超导性仍然很强(Tc约为55 K),所以我们的结果排除了磁共振峰和声子作为高Tc超导性主要成因的可能性。另一方面,这个宽泛的背景是铜氧平面的一个普遍特性,并且为束缚电子的“胶水”提供了一个很好的候选特征。