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通过红外光谱法获得的K掺杂BaFe[化学式:见原文]As[化学式:见原文]的掺杂依赖性超导物理量。

Doping-dependent superconducting physical quantities of K-doped BaFe[Formula: see text]As[Formula: see text] obtained through infrared spectroscopy.

作者信息

Lee Seokbae, Seo Yu-Seong, Roh Seulki, Song Dongjoon, Eisaki Hiroshi, Hwang Jungseek

机构信息

Department of Physics, Sungkyunkwan University, Suwon, Gyeonggi-do 16419 Republic of Korea.

National Institute of Advanced Industrial Science and Technology, Tsukuba, 305-8568 Japan.

出版信息

Sci Rep. 2022 Nov 19;12(1):19950. doi: 10.1038/s41598-022-24520-y.

DOI:10.1038/s41598-022-24520-y
PMID:36402847
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC9675795/
Abstract

We investigated four single crystals of K-doped BaFe[Formula: see text]As[Formula: see text] (Ba-122), Ba[Formula: see text]K[Formula: see text]Fe[Formula: see text]As[Formula: see text] with [Formula: see text] 0.29, 0.36, 0.40, and 0.51, using infrared spectroscopy. We explored a wide variety of doping levels, from under- to overdoped. We obtained the superfluid plasma frequencies ([Formula: see text]) and corresponding London penetration depths ([Formula: see text]) from the measured optical conductivity spectra. We also extracted the electron-boson spectral density (EBSD) functions using a two-parallel charge transport channel approach in the superconducting (SC) state. From the extracted EBSD functions, the maximum SC transition temperatures ([Formula: see text]) were determined using a generalized McMillan formula and the SC coherence lengths ([Formula: see text]) were calculated using the timescales encoded in the EBSD functions and reported Fermi velocities. We identified some similarities and differences in the doping-dependent SC quantities between the K-doped Ba-122 and the hole-doped cuprates. We expect that the various SC quantities obtained across the wide doping range will provide helpful information for establishing the microscopic pairing mechanism in Fe-pnictide superconductors.

摘要

我们使用红外光谱研究了四种钾掺杂的BaFe₂As₂(Ba-122)单晶,即Ba₂KₓFe₂As₂(x = 0.29、0.36、0.40和0.51)。我们探索了从欠掺杂到过掺杂的各种掺杂水平。我们从测量的光导率光谱中获得了超流等离子体频率(ωₚ)和相应的伦敦穿透深度(λ)。我们还在超导(SC)状态下使用双平行电荷传输通道方法提取了电子-玻色子光谱密度(EBSD)函数。根据提取的EBSD函数,使用广义麦克米兰公式确定了最大超导转变温度(Tₘₐₓ),并使用EBSD函数中编码的时间尺度和报道的费米速度计算了超导相干长度(ξ)。我们确定了钾掺杂的Ba-122和空穴掺杂的铜酸盐之间在掺杂依赖的超导量方面的一些异同。我们期望在宽掺杂范围内获得的各种超导量将为建立铁基超导体中的微观配对机制提供有用信息。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8bb6/9675795/3c1c96cf8653/41598_2022_24520_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8bb6/9675795/3f2de5b6e07f/41598_2022_24520_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8bb6/9675795/3b1573aaa004/41598_2022_24520_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8bb6/9675795/39996bea38b1/41598_2022_24520_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8bb6/9675795/3c1c96cf8653/41598_2022_24520_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8bb6/9675795/3f2de5b6e07f/41598_2022_24520_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8bb6/9675795/3b1573aaa004/41598_2022_24520_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8bb6/9675795/39996bea38b1/41598_2022_24520_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8bb6/9675795/3c1c96cf8653/41598_2022_24520_Fig4_HTML.jpg

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本文引用的文献

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Nature. 2022 Jan;601(7891):35-44. doi: 10.1038/s41586-021-04073-2. Epub 2022 Jan 5.
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Superconducting coherence length of hole-doped cuprates obtained from electron-boson spectral density function.从电子-玻色子谱密度函数获得的空穴掺杂铜酸盐的超导相干长度。
Sci Rep. 2021 Jun 3;11(1):11668. doi: 10.1038/s41598-021-91163-w.
3
Analysis of optical data using extended Drude model and generalized Allen's formulas.使用扩展德鲁德模型和广义艾伦公式对光学数据进行分析。
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Electron-boson spectral density function of correlated multiband systems obtained from optical data: Ba0.6K0.4Fe2As2 and LiFeAs.
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Reverse process of usual optical analysis of boson-exchange superconductors: impurity effects on s- and d-wave superconductors.玻色子交换超导体常规光学分析的逆过程:杂质对s波和d波超导体的影响。
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Electron-boson spectral density of LiFeAs obtained from optical data.从光学数据获得的LiFeAs的电子-玻色子谱密度。
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Normal-state charge dynamics in doped BaFe₂As₂: roles of doping and necessary ingredients for superconductivity.掺杂BaFe₂As₂中的正常态电荷动力学:掺杂的作用及超导的必要成分
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