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欧盟委员会玛丽娜二号研究结果:第二部分——天然放射性物质排放的影响

Results of the European Commission Marina II study: part II--effects of discharges of naturally occurring radioactive material.

作者信息

Betti M, Aldave de las Heras L, Janssens A, Henrich E, Hunter G, Gerchikov M, Dutton M, van Weers A W, Nielsen S, Simmonds J, Bexon A, Sazykina T

机构信息

European Commission, Joint Research Centre, Institute for Transuranium Elements, P.O. Box 2340, 76125 Karlsruhe, Germany.

出版信息

J Environ Radioact. 2004;74(1-3):255-77. doi: 10.1016/j.jenvrad.2004.01.021.

Abstract

Enhanced levels of naturally occurring radioactive materials (NORM) are produced through various industrial operations and may lead to discharges to the marine environment. A recent study, called MARINA II, carried out for the European Commission considered discharges of radionuclides from the NORM industries to north European marine waters and their consequences. There are two main sources that were considered in the study. The use of phosphogypsum during the production of phosphoric acid by the fertiliser industry and the pumping of oil and gas from the continental shelf in the North Sea which produces large quantities of water contaminated with enhanced levels of naturally occurring radionuclides. Discharges of alpha emitting radionuclides from these two industries have contributed significantly to the total input of alpha emitters to north European waters over the period 1981-2000 (data were not available prior to 1981). Discharges due to the use of phosphogypsum have declined since the early 1990s and are now very low. Discharges from the oil and gas industries stabilised in the second half of the 1990s and are now the major contributor to alpha discharges to the region. As most European countries do not report discharges of radioactivity with the water produced during extraction, there is considerable uncertainty in the discharges used in the study. The impact of the discharges has been estimated both in terms of the effect on non-human biota and the radiological impact for people. In the 1980s the radiation dose rates to marine biota in the region around a phosphate plant on the north-west coast of England were as high due to the discharges from the phosphate plant as those near to the Sellafield reprocessing plant due to its discharges. In recent years the additional dose to marine biota in this region due to the past NORM discharges is of the same order of magnitude as the natural background. The collective dose rate was estimated to determine the radiological impact on people. The peak collective dose rate from the NORM industries occurred in 1984 and was just over 600 manSv y(-1). The collective dose rate fell with time as discharges from the phosphate industry reduced and was estimated as under 200 manSv y(-1) in 2000.

摘要

各种工业活动会产生自然产生的放射性物质(NORM)水平升高的情况,这可能导致向海洋环境排放。最近为欧盟委员会开展的一项名为“MARINA II”的研究,考量了NORM行业向北欧海域排放放射性核素的情况及其后果。该研究考虑了两个主要来源。化肥行业在生产磷酸过程中使用磷石膏,以及从北海大陆架开采石油和天然气,这会产生大量被自然产生的放射性核素水平升高所污染的水。在1981年至2000年期间,这两个行业排放的发射α粒子的放射性核素对北欧水域α发射体的总输入量贡献显著(1981年之前没有相关数据)。自20世纪90年代初以来,因使用磷石膏导致的排放有所下降,目前非常低。石油和天然气行业的排放于20世纪90年代后半期趋于稳定,现在是该地区α排放的主要贡献者。由于大多数欧洲国家不报告开采过程中产生的水中放射性物质的排放情况,该研究中所使用的排放量存在相当大的不确定性。已从对非人类生物群的影响以及对人类的辐射影响这两方面估算了排放的影响。在20世纪80年代,英格兰西北海岸一家磷酸盐工厂周围地区,由于该磷酸盐工厂的排放,海洋生物群受到的辐射剂量率与因塞拉菲尔德后处理厂排放而受到的辐射剂量率一样高。近年来,由于过去NORM排放给该地区海洋生物群带来的额外剂量与自然本底处于同一数量级。通过估算集体剂量率来确定对人类的辐射影响。NORM行业的集体剂量率峰值出现在1984年,略高于600人希沃特/年。随着磷酸盐行业排放的减少,集体剂量率随时间下降,2000年估计低于200人希沃特/年。

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