Asmi Ari J, Pirjola Liisa H, Kulmala Markku
University of Helsinki, Department of Physical Sciences, Helsinki, Finland.
Scand J Work Environ Health. 2004;30 Suppl 2:63-72.
This study attempted to simulate indoor concentrations and the indoor-to-outdoor (I:O) number concentration ratios of aerosol particles in the submicron size range.
The developed model used size-segregated outdoor number concentrations of particles as inputs and produced the indoor aerosol size spectrum. It covered all the major dynamic processes associated with the indoor aerosol concentration: transport and filtration in the air exchange system, deposition, coagulation, nucleation, condensation, and indoor sources. The model results were compared with measured particle concentrations. Numerous sensitivity analyses were also made for testing the effect of different dynamic processes on the model results. No indoor particle sources were considered in the sensitivity simulations.
Changes in the air exchange rate had the strongest effect on the simulated I:O ratios of particle number concentrations. Filtration in the air exchange system also had a large effect on the indoor concentrations. Deposition did not significantly change the particle number concentrations within a realistic range of turbulence intensity indoors and the temperature differences between the ambient air and surfaces. Coagulation affected only the smallest particle size ranges. Condensation and nucleation had potentially large effects on the particle size spectrum.
The model reproduced the measured I:O ratios of fine and ultrafine particle concentrations with reasonable accuracy. The model can be a valuable tool with which to estimate the I:O ratios for human exposure assessment.
本研究试图模拟亚微米尺寸范围内气溶胶颗粒的室内浓度以及室内与室外(I:O)数量浓度比。
所开发的模型将按粒径分类的室外颗粒数量浓度作为输入,并生成室内气溶胶粒径谱。它涵盖了与室内气溶胶浓度相关的所有主要动态过程:空气交换系统中的传输和过滤、沉积、凝聚、成核、凝结以及室内源。将模型结果与实测颗粒浓度进行了比较。还进行了大量敏感性分析,以测试不同动态过程对模型结果的影响。在敏感性模拟中未考虑室内颗粒源。
空气交换率的变化对模拟的颗粒数量浓度I:O比影响最大。空气交换系统中的过滤对室内浓度也有很大影响。在室内实际湍流强度范围以及环境空气与表面之间的温差范围内,沉积对颗粒数量浓度没有显著影响。凝聚仅影响最小粒径范围。凝结和成核对粒径谱可能有很大影响。
该模型以合理的精度再现了实测的细颗粒和超细颗粒浓度的I:O比。该模型可成为估算用于人体暴露评估的I:O比的宝贵工具。