Veselovskii Igor, Kolgotin Alexei, Müller Detlef, Whiteman David N
Physics Instrumentation Center, Troitsk, Moscow Region 142190, Russia.
Appl Opt. 2005 Sep 1;44(25):5292-303. doi: 10.1364/ao.44.005292.
The multiwavelength Raman lidar technique in combination with sophisticated inversion algorithms has been recognized as a new tool for deriving information about the microphysical properties of atmospheric aerosols. The input optical parameter sets, provided by respective aerosol Raman lidars, are at the theoretical lower limit at which these inversion algorithms work properly. For that reason there is ongoing intense discussion of the accuracy of these inversion methods and the possibility of simultaneous retrieval of the particle size distribution and the complex refractive index. We present results of the eigenvalue analysis, used to study the information content of multiwavelength lidar data with respect to microphysical particle properties. Such an analysis provides, on a rather mathematical basis, more insight into the limitations of these inversion algorithms regarding the accuracy of the retrieved parameters. We show that the effective radius may be retrieved to 50% accuracy and the real and imaginary part of the complex refractive index to +/- 0.05 and +/- 0.005i, if the imaginary part is < 0.02i. These results are in accordance with the classic approach of simulation studies with synthetic particle size distributions. Major difficulties are found with a particle effective radius of < 0.15 microm. In that case the complex refractive index may not be derived with sufficient accuracy. The eigenvalue analysis also shows that the accuracy of the derived parameters degrades if the imaginary part is > 0.02i. Furthermore it shows the importance of the simultaneous use of backscatter and extinction coefficients for the retrieval of microphysical parameters.
多波长拉曼激光雷达技术与先进的反演算法相结合,已被公认为是一种获取大气气溶胶微物理特性信息的新工具。由各自的气溶胶拉曼激光雷达提供的输入光学参数集处于这些反演算法正常工作的理论下限。因此,关于这些反演方法的准确性以及同时反演粒径分布和复折射率的可能性,正在进行激烈的讨论。我们展示了特征值分析的结果,该分析用于研究多波长激光雷达数据关于微物理粒子特性的信息含量。这样的分析在相当数学的基础上,能更深入地了解这些反演算法在反演参数准确性方面的局限性。我们表明,如果虚部<0.02i,有效半径可以以50%的精度反演出来,复折射率的实部和虚部分别可以反演到±0.05和±0.005i。这些结果与用合成粒径分布进行模拟研究的经典方法一致。当粒子有效半径<0.15微米时会发现主要困难。在这种情况下,复折射率可能无法以足够的精度推导出来。特征值分析还表明,如果虚部>0.02i,推导参数的准确性会下降。此外,它还表明了同时使用后向散射系数和消光系数来反演微物理参数的重要性。