Müller D, Wandinger U, Ansmann A
Institute for Tropospheric Research, Permoserstrasse 15, 04318 Leipzig, Germany.
Appl Opt. 1999 Apr 20;38(12):2358-68. doi: 10.1364/ao.38.002358.
A sensitivity study with an inversion scheme that permits one to retrieve physical parameters of tropospheric particle size distributions, e.g., effective radius, volume, surface-area, and number concentrations, as well as the mean complex refractive index from backscatter and extinction coefficients at multiple wavelengths is presented. The optical data for the analysis are derived from Mie-scattering calculations for monomodal and bimodal logarithmic-normal distributions in the particle size range between 0.01 and 10 microm. The complex refractive index is taken between 1.33 and 1.8 in the real part and between 0 and 0.1 in the imaginary part. The choice of these parameters takes account of properties of optically active atmospheric particles. The wavelengths were chosen at 355, 400, 532, 710, 800, and 1064 nm for the backscatter and at 355 and 532 nm for the extinction data, which are the available wavelengths of the two lidar systems at the Institute for Tropospheric Research. Cases of erroneous optical data of the order of as much as 20%, an unknown refractive index, which may also be wavelength and size dependent, as well as the a priori unknown modality of the particle size distribution were considered. It is shown that both extinction channels are necessary for determining the above-mentioned parameters within reasonable limits, i.e., effective radius, surface-area, and volume concentrations to an accuracy of +/-50%, the real part of the complex refractive index to +/-0.1, and the imaginary part to +/-50%. The number concentration may have errors larger than 50%. The overall performance of the inversion scheme permits the evaluation of experimental data on a routine basis.
本文介绍了一项灵敏度研究,该研究采用了一种反演方案,该方案能够从多个波长的后向散射和消光系数中反演对流层粒子粒径分布的物理参数,例如有效半径、体积、表面积和数浓度,以及平均复折射率。用于分析的光学数据源自对粒径范围在0.01至10微米之间的单峰和双峰对数正态分布进行的米氏散射计算。复折射率的实部取值范围为1.33至1.8,虚部取值范围为0至0.1。这些参数的选择考虑了光学活性大气粒子的特性。后向散射数据的波长选择为355、400、532、710、800和1064纳米,消光数据的波长选择为355和532纳米,这是对流层研究所两个激光雷达系统可获得的波长。考虑了光学数据误差高达20%的情况、未知的折射率(其也可能与波长和粒径有关)以及粒径分布的先验未知模态。结果表明,两个消光通道对于在合理范围内确定上述参数是必要的,即有效半径、表面积和体积浓度的精度为±50%,复折射率实部的精度为±0.1,虚部的精度为±50%。数浓度的误差可能大于50%。反演方案的整体性能允许对实验数据进行常规评估。