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Heterodyne spectral interferometry for multidimensional nonlinear spectroscopy of individual quantum systems.

作者信息

Langbein Wolfgang, Patton Brian

机构信息

School of Physics and Astronomy, Cardiff University, Cardiff CF24 3YB, UK.

出版信息

Opt Lett. 2006 Apr 15;31(8):1151-3. doi: 10.1364/ol.31.001151.

DOI:10.1364/ol.31.001151
PMID:16625933
Abstract

A novel implementation of transient nonlinear spectroscopy is presented that allows the study of the transient nonlinear polarization emitted from individual electronic transitions. Both the amplitude and the phase of the polarization are retrieved, permitting the implementation of multidimensional spectroscopy in the excitation pulse delays. The technique is shown to detect mutual coherent coupling in a group of individual, localized excitonic transitions.

摘要

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