• 文献检索
  • 文档翻译
  • 深度研究
  • 学术资讯
  • Suppr Zotero 插件Zotero 插件
  • 邀请有礼
  • 套餐&价格
  • 历史记录
应用&插件
Suppr Zotero 插件Zotero 插件浏览器插件Mac 客户端Windows 客户端微信小程序
定价
高级版会员购买积分包购买API积分包
服务
文献检索文档翻译深度研究API 文档MCP 服务
关于我们
关于 Suppr公司介绍联系我们用户协议隐私条款
关注我们

Suppr 超能文献

核心技术专利：CN118964589B侵权必究
粤ICP备2023148730 号-1Suppr @ 2026

文献检索

告别复杂PubMed语法，用中文像聊天一样搜索，搜遍4000万医学文献。AI智能推荐，让科研检索更轻松。

立即免费搜索

文件翻译

保留排版，准确专业，支持PDF/Word/PPT等文件格式，支持 12+语言互译。

免费翻译文档

深度研究

AI帮你快速写综述，25分钟生成高质量综述，智能提取关键信息，辅助科研写作。

立即免费体验

半导体纳米结构的多维相干光谱学进展。

Advances in multi-dimensional coherent spectroscopy of semiconductor nanostructures.

作者信息

Moody Galan, Cundiff Steven T

机构信息

Applied Physics Division, National Institute of Standards & Technology, Boulder, CO, USA.

Department of Physics, University of Michigan, Ann Arbor, MI, USA.

出版信息

Adv Phys X. 2017;2(3):641-674. doi: 10.1080/23746149.2017.1346482. Epub 2017 Jul 17.

DOI:10.1080/23746149.2017.1346482
PMID:28894306
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC5590666/
Abstract

Multi-dimensional coherent spectroscopy (MDCS) has become an extremely versatile and sensitive technique for elucidating the structure, composition, and dynamics of condensed matter, atomic, and molecular systems. The appeal of MDCS lies in its ability to resolve both individual-emitter and ensemble-averaged dynamics of optically created excitations in disordered systems. When applied to semiconductors, MDCS enables unambiguous separation of homogeneous and inhomogeneous contributions to the optical linewidth, pinpoints the nature of coupling between resonances, and reveals signatures of many-body interactions. In this review, we discuss the implementation of MDCS to measure the nonlinear optical response of excitonic transitions in semiconductor nanostructures. Capabilities of the technique are illustrated with recent experimental studies that advance our understanding of optical decoherence and dissipation, energy transfer, and many-body phenomena in quantum dots and quantum wells, semiconductor microcavities, layered semiconductors, and photovoltaic materials.

摘要

多维相干光谱学（MDCS）已成为一种极为通用且灵敏的技术，用于阐明凝聚态物质、原子和分子系统的结构、组成及动力学。MDCS的吸引力在于它能够分辨无序系统中光学产生的激发的单个发射体动力学和系综平均动力学。当应用于半导体时，MDCS能够明确分离均匀和非均匀对光学线宽的贡献，确定共振之间耦合的性质，并揭示多体相互作用的特征。在本综述中，我们讨论了MDCS用于测量半导体纳米结构中激子跃迁的非线性光学响应的实现。该技术的能力通过最近的实验研究得到了说明，这些研究推进了我们对量子点和量子阱、半导体微腔、层状半导体及光伏材料中的光学退相干和耗散、能量转移及多体现象的理解。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/2f0fde807cdb/nihms899073f13.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/79d79414ef8a/nihms899073f1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/a8cde2921165/nihms899073f2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/1204b9a42622/nihms899073f3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/0f9d45b65743/nihms899073f4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/bde46f9b614e/nihms899073f5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/a36d850dfe13/nihms899073f6.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/0aee08221f92/nihms899073f7.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/74721107540d/nihms899073f8.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/81ea10a50719/nihms899073f9.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/f0c7a06bfdda/nihms899073f10.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/f883a7d7b58f/nihms899073f11.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/06b9f30db0c4/nihms899073f12.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/2f0fde807cdb/nihms899073f13.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/79d79414ef8a/nihms899073f1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/a8cde2921165/nihms899073f2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/1204b9a42622/nihms899073f3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/0f9d45b65743/nihms899073f4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/bde46f9b614e/nihms899073f5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/a36d850dfe13/nihms899073f6.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/0aee08221f92/nihms899073f7.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/74721107540d/nihms899073f8.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/81ea10a50719/nihms899073f9.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/f0c7a06bfdda/nihms899073f10.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/f883a7d7b58f/nihms899073f11.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/06b9f30db0c4/nihms899073f12.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/79ab/5590666/2f0fde807cdb/nihms899073f13.jpg

相似文献

1
Advances in multi-dimensional coherent spectroscopy of semiconductor nanostructures.半导体纳米结构的多维相干光谱学进展。
Adv Phys X. 2017;2(3):641-674. doi: 10.1080/23746149.2017.1346482. Epub 2017 Jul 17.
2
Optical two-dimensional fourier transform spectroscopy of semiconductor quantum wells.半导体量子阱的光学二维傅里叶变换光谱学。
Acc Chem Res. 2009 Sep 15;42(9):1423-32. doi: 10.1021/ar9000636.
3
Ultrafast near-field spectroscopy of single semiconductor quantum dots.单半导体量子点的超快近场光谱学
Philos Trans A Math Phys Eng Sci. 2004 Apr 15;362(1817):861-79. doi: 10.1098/rsta.2003.1353.
4
Optical coherence and collective phenomena in nanostructures.纳米结构中的光学相干与集体现象。
J Phys Condens Matter. 2007 Jul 25;19(29):290301. doi: 10.1088/0953-8984/19/29/290301. Epub 2007 Jun 11.
5
Transient coherent nonlinear spectroscopy of single quantum dots.单量子点的瞬态相干非线性光谱学
J Phys Condens Matter. 2007 Jul 25;19(29):295203. doi: 10.1088/0953-8984/19/29/295203. Epub 2007 Jun 11.
6
Nonlinear plasmon-exciton coupling enhances sum-frequency generation from a hybrid metal/semiconductor nanostructure.非线性等离子体激元-激子耦合增强了混合金属/半导体纳米结构的和频产生。
Nat Commun. 2020 Mar 19;11(1):1464. doi: 10.1038/s41467-020-15232-w.
7
Up on the Jaynes-Cummings ladder of a quantum-dot/microcavity system.在量子点/微腔系统的 Jaynes-Cummings 阶梯上。
Nat Mater. 2010 Apr;9(4):304-8. doi: 10.1038/nmat2717. Epub 2010 Mar 7.
8
Separating homogeneous and inhomogeneous line widths of heavy- and light-hole excitons in weakly disordered semiconductor quantum wells. 弱无序半导体量子阱中重空穴和轻空穴激子的同质和非同质线宽分离。
J Phys Chem B. 2011 May 12;115(18):5365-71. doi: 10.1021/jp109408s. Epub 2011 Mar 9.
9
Simultaneous Existence of Confined and Delocalized Vibrational Modes in Colloidal Quantum Dots.胶体量子点中受限和离域振动模式的同时存在。
J Phys Chem Lett. 2019 Oct 17;10(20):6144-6150. doi: 10.1021/acs.jpclett.9b02474. Epub 2019 Oct 1.
10
Ultrafast dynamics of many-body processes and fundamental quantum mechanical phenomena in semiconductors.半导体中多体过程和基本量子力学现象的超快动力学。
Proc Natl Acad Sci U S A. 2000 Mar 14;97(6):2437-44. doi: 10.1073/pnas.97.6.2437.

引用本文的文献

1
Dephasing of InAs quantum dot -shell excitons studied using two-dimensional coherent spectroscopy.利用二维相干光谱研究砷化铟量子点壳层激子的退相
Phys Rev B. 2018 Nov;98(19). doi: 10.1103/PhysRevB.98.195304.
2
Development of Two-Dimensional Electronic-Vibrational Sum Frequency Generation (2D-EVSFG) for Vibronic and Solvent Couplings of Molecules at Interfaces and Surfaces.用于界面和表面分子的电子振动耦合及溶剂耦合的二维电子振动和频产生（2D-EVSFG）技术的发展
ACS Phys Chem Au. 2023 Apr 25;3(4):374-385. doi: 10.1021/acsphyschemau.3c00011. eCollection 2023 Jul 26.
3
Persistent coherence of quantum superpositions in an optimally doped cuprate revealed by 2D spectroscopy.

本文引用的文献

1
Exciton Dynamics in Monolayer Transition Metal Dichalcogenides.单层过渡金属二硫属化物中的激子动力学
J Opt Soc Am B. 2016 Jul 1;33(7):C39-C49. doi: 10.1364/JOSAB.33.000C39. Epub 2016 Apr 19.
2
Neutral and charged inter-valley biexcitons in monolayer MoSe.单层 MoSe 中的中性和带电谷间双激子
Nat Commun. 2017 Jun 28;8:15552. doi: 10.1038/ncomms15552.
3
Controlling quantum-beating signals in 2D electronic spectra by packing synthetic heterodimers on single-walled carbon nanotubes.通过将合成杂二聚体组装在单壁碳纳米管上来控制二维电子光谱中的量子拍频信号。
二维光谱揭示最佳掺杂铜酸盐中量子叠加态的持久相干性。
Sci Adv. 2020 Feb 28;6(9):eaaw9932. doi: 10.1126/sciadv.aaw9932. eCollection 2020 Feb.
Nat Chem. 2017 Feb 21;9(3):219-225. doi: 10.1038/nchem.2729.
4
Coherent Control of the Exciton-Biexciton System in an InAs Self-Assembled Quantum Dot Ensemble.InAs自组装量子点系综中激子-双激子系统的相干控制
Phys Rev Lett. 2016 Oct 7;117(15):157402. doi: 10.1103/PhysRevLett.117.157402. Epub 2016 Oct 6.
5
Revealing and Characterizing Dark Excitons through Coherent Multidimensional Spectroscopy.通过相干多维光谱揭示和表征暗激子
Phys Rev Lett. 2016 Aug 26;117(9):097401. doi: 10.1103/PhysRevLett.117.097401. Epub 2016 Aug 23.
6
Broadband 7-fs diffractive-optic-based 2D electronic spectroscopy using hollow-core fiber compression.基于空心光纤压缩的宽带7飞秒衍射光学二维电子光谱学。
Opt Express. 2016 Sep 5;24(18):20781-91. doi: 10.1364/OE.24.020781.
7
Radiatively Limited Dephasing and Exciton Dynamics in MoSe2 Monolayers Revealed with Four-Wave Mixing Microscopy.四波混频显微镜揭示 MoSe2 单层中的辐射限制退相和激子动力学。
Nano Lett. 2016 Sep 14;16(9):5333-9. doi: 10.1021/acs.nanolett.6b01060. Epub 2016 Aug 22.
8
Coherent and Incoherent Coupling Dynamics between Neutral and Charged Excitons in Monolayer MoSe2.单层 MoSe2 中中性激子和带电激子的相干和非相干耦合动力学。
Nano Lett. 2016 Aug 10;16(8):5109-13. doi: 10.1021/acs.nanolett.6b02041. Epub 2016 Jul 22.
9
Ultrafast Exciton Hopping Observed in Bare Semiconducting Carbon Nanotube Thin Films with Two-Dimensional White-Light Spectroscopy.利用二维白光光谱在裸半导体碳纳米管薄膜中观测到超快激子跳跃
J Phys Chem Lett. 2016 Jun 2;7(11):2024-31. doi: 10.1021/acs.jpclett.6b00650. Epub 2016 May 19.
10
Optical Coherence in Atomic-Monolayer Transition-Metal Dichalcogenides Limited by Electron-Phonon Interactions.原子层过渡金属二卤族化合物中受电子-声子相互作用限制的光学相干性。
Phys Rev Lett. 2016 Mar 25;116(12):127402. doi: 10.1103/PhysRevLett.116.127402.