Zhu Dongwei, Wang Yan, Pang Yan, Liu Ang, Guo Jian, Bouwman Carolien A, West Clive E, van Breemen Richard B
College of Pharmacy, University of Illinois at Chicago, Chicago, IL 60612, USA.
Rapid Commun Mass Spectrom. 2006;20(16):2427-32. doi: 10.1002/rcm.2601.
Among more than 50 provitamin carotenoids, beta-carotene is the most metabolically active source of retinol. Despite diets rich in fruits and vegetables containing beta-carotene, vitamin A deficiency is the leading cause of blindness and childhood mortality in developing countries. In addition, the uncertainty of beta-carotene bioconversion into vitamin A suggests that new data are needed to update the nutritional guidelines in developed countries. Previously, we reported the development of a carotene/retinol plateau isotopic enrichment method (CarRet PIE) for the determination of beta-carotene bioavailability and bioconversion into retinol, which utilizes positive ion atmospheric pressure chemical ionization (APCI) liquid chromatography/mass spectrometry (LC/MS). While seeking to validate the CarRet PIE using a mass balance approach requiring fecal measurements of beta-carotene and retinol, interference was encountered that required substantial modifications of the LC/MS assay. Here we report a new LC/MS assay that is based on the detection of molecular anions of beta-carotene using negative ion APCI with a reversed-phase C30 column for HPLC separation. Sample preparation required saponification to eliminate interfering triglycerides. The limit of detection (LOD) of beta-carotene was 0.25 pmol calculated on the basis of an injection of 20 microL of 0.0125 microM beta-carotene, and the limit of quantitation (LOQ) was 1.0 pmol based on the injection of 20 microL of 0.050 microM beta-carotene. The linear range was 1.1 to 2179 pmol on-column. The wide linear range and low LOD and LOQ of this assay facilitated the sensitive and selective quantitative analysis of beta-carotene in both serum and fecal samples in support of an on-going clinical investigation of beta-carotene bioavailability and bioconversion into vitamin A.
在50多种维生素原类胡萝卜素中,β-胡萝卜素是视黄醇代谢活性最高的来源。尽管饮食中富含含有β-胡萝卜素的水果和蔬菜,但维生素A缺乏仍是发展中国家失明和儿童死亡的主要原因。此外,β-胡萝卜素生物转化为维生素A的不确定性表明,需要新的数据来更新发达国家的营养指南。此前,我们报道了一种用于测定β-胡萝卜素生物利用度及其向视黄醇生物转化的胡萝卜素/视黄醇平台同位素富集方法(CarRet PIE),该方法利用正离子大气压化学电离(APCI)液相色谱/质谱(LC/MS)。在试图使用需要对粪便中的β-胡萝卜素和视黄醇进行测量的质量平衡方法验证CarRet PIE时,遇到了干扰,这需要对LC/MS分析进行大量修改。在此,我们报告一种新的LC/MS分析方法,该方法基于使用负离子APCI和反相C30柱进行HPLC分离来检测β-胡萝卜素的分子阴离子。样品制备需要皂化以消除干扰性甘油三酯。基于进样20 μL 0.0125 μM的β-胡萝卜素计算,β-胡萝卜素的检测限(LOD)为0.25 pmol,基于进样20 μL 0.050 μM的β-胡萝卜素计算,定量限(LOQ)为1.0 pmol。柱上线性范围为1.1至2179 pmol。该分析方法的宽线性范围以及低LOD和LOQ有助于对血清和粪便样品中的β-胡萝卜素进行灵敏且选择性的定量分析,以支持正在进行的关于β-胡萝卜素生物利用度及其向维生素A生物转化的临床研究。