Doiron-Leyraud Nicolas, Proust Cyril, LeBoeuf David, Levallois Julien, Bonnemaison Jean-Baptiste, Liang Ruixing, Bonn D A, Hardy W N, Taillefer Louis
Département de physique and RQMP, Université de Sherbrooke, Sherbrooke, Canada J1K 2R1.
Nature. 2007 May 31;447(7144):565-8. doi: 10.1038/nature05872.
Despite twenty years of research, the phase diagram of high-transition-temperature superconductors remains enigmatic. A central issue is the origin of the differences in the physical properties of these copper oxides doped to opposite sides of the superconducting region. In the overdoped regime, the material behaves as a reasonably conventional metal, with a large Fermi surface. The underdoped regime, however, is highly anomalous and appears to have no coherent Fermi surface, but only disconnected 'Fermi arcs'. The fundamental question, then, is whether underdoped copper oxides have a Fermi surface, and if so, whether it is topologically different from that seen in the overdoped regime. Here we report the observation of quantum oscillations in the electrical resistance of the oxygen-ordered copper oxide YBa2Cu3O6.5, establishing the existence of a well-defined Fermi surface in the ground state of underdoped copper oxides, once superconductivity is suppressed by a magnetic field. The low oscillation frequency reveals a Fermi surface made of small pockets, in contrast to the large cylinder characteristic of the overdoped regime. Two possible interpretations are discussed: either a small pocket is part of the band structure specific to YBa2Cu3O6.5 or small pockets arise from a topological change at a critical point in the phase diagram. Our understanding of high-transition-temperature (high-T(c)) superconductors will depend critically on which of these two interpretations proves to be correct.
尽管经过了二十年的研究,但高温超导材料的相图仍然是个谜。一个核心问题是,这些掺杂到超导区域两侧的铜氧化物在物理性质上存在差异的根源。在过掺杂状态下,材料表现得像一种相当传统的金属,具有很大的费米面。然而,欠掺杂状态却非常反常,似乎没有连贯的费米面,只有不相连的“费米弧”。那么,根本问题在于,欠掺杂的铜氧化物是否存在费米面,如果存在,其拓扑结构是否与过掺杂状态下的不同。在此,我们报告了对氧有序铜氧化物YBa2Cu3O6.5电阻中的量子振荡的观测结果,证实了在磁场抑制超导性后,欠掺杂铜氧化物基态中存在明确的费米面。低振荡频率揭示出一个由小口袋状构成的费米面,这与过掺杂状态下的大圆柱状特征形成对比。文中讨论了两种可能的解释:要么小口袋状是YBa2Cu3O6.5特有的能带结构的一部分,要么小口袋状是相图中临界点处拓扑变化的结果。我们对高温超导材料的理解将严重依赖于这两种解释中哪一种被证明是正确的。