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气象条件和颗粒物对中国济南视程障碍的影响。

Influence of meteorological conditions and particulate matter on visual range impairment in Jinan, China.

作者信息

Yang Ling-Xiao, Wang Dong-Cheng, Cheng Shu-Hui, Wang Zhe, Zhou Yang, Zhou Xue-Hua, Wang Wen-Xing

机构信息

Environment Research Institute, Shandong University, Jinan, PR China.

出版信息

Sci Total Environ. 2007 Sep 20;383(1-3):164-73. doi: 10.1016/j.scitotenv.2007.04.042. Epub 2007 Jun 13.

Abstract

To understand the influence of aerosol particles and meteorological conditions on visual range in Jinan, the capital of Shandong Province, China, PM(2.5) and PM(10) samples were collected from November 2004 to September 2005. The mass concentrations of PM(2.5) and PM(10), concentrations of water-soluble ions in PM(2.5) and concentrations of black carbon (BC) in the atmosphere were analyzed. The decrease of visual range in Jinan results from the combined influence of PM(2.5), PM(10) and meteorological conditions. For the period studied, the average light extinction coefficient, b(ext), which was estimated from an equation developed by the IMPROVE network was 292 Mm(-1). Ammonium sulfate was the major contributor to visual range impairment, accounting for 41%, while ammonium nitrate, particulate organic matter (POM) and BC made comparable contributions accounting for 20%, 22% and 18%, respectively. This highlights the significance of secondary particles ((NH(4))(2)SO(4), NH(4)NO(3), POM) in visual range impairment in Jinan. The data from this study are also compared with the long-term variations of visual range in Jinan from 1961 to 2005.

摘要

为了解气溶胶颗粒和气象条件对中国山东省省会济南市能见度的影响,于2004年11月至2005年9月采集了PM(2.5)和PM(10)样本。分析了PM(2.5)和PM(10)的质量浓度、PM(2.5)中水溶性离子的浓度以及大气中黑碳(BC)的浓度。济南市能见度的降低是PM(2.5)、PM(10)和气象条件共同影响的结果。在所研究的时间段内,根据IMPROVE网络开发的一个方程估算出的平均光消光系数b(ext)为292 Mm(-1)。硫酸铵是造成能见度降低的主要因素,占41%,而硝酸铵、颗粒有机物(POM)和黑碳的贡献相当,分别占20%、22%和18%。这突出了二次颗粒物((NH(4))(2)SO(4)、NH(4)NO(3)、POM)在济南市能见度降低中的重要性。本研究的数据还与1961年至2005年济南市能见度长期变化情况进行了比较。

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