Ray Krishanu, Chowdhury Mustafa H, Lakowicz Joseph R
Center for Fluorescence Spectroscopy, Department of Biochemistry and Molecular Biology, University of Maryland School of Medicine, Baltimore, MD 21201, USA.
Anal Chem. 2007 Sep 1;79(17):6480-7. doi: 10.1021/ac071363l. Epub 2007 Aug 8.
Particulate aluminum films of varied thicknesses were deposited on quartz substrates by thermal evaporation. These nanostructured substrates were characterized by scanning electron microscopy (SEM). With the increase of aluminum thickness, the films progress from articulate toward smooth surfaces as observed by SEM images. To date, metal-enhanced fluorescence (MEF) has primarily been observed in the visible - NIR wavelength region using silver or gold island films or roughened surfaces. We now show that fluorescence could also be enhanced in the ultraviolet-blue region of the spectrum using nanostructured aluminum films. Two probes, one in the ultraviolet and another one in the blue spectral region, have been chosen for the present study. We observed increased emission, decrease in fluorescence lifetime, and increase in photostability of a DNA base analogue 2-aminopurine and a coumarin derivative (7-HC) in 10-nm spin-casted poly(vinyl alcohol) film on Al nanostructured surfaces. The fluorescence enhancement factor depends on the thickness of the Al films as the size of the nanostructures formed varies with Al thickness. Both probes showed increased photostability near aluminum nanostructured substrates, which is consistent with the shorter lifetime. Our preliminary studies indicate that Al nanostructured substrates can potentially find widespread use in MEF applications particularly in the UV-blue spectral regime. Furthermore, these Al nanostructured substrates are very stable in buffers that contain chloride salts compared to usual silver colloid-based substrates for MEF, thus furthering the usefulness of these Al-based substrates in many biological assays where high concentration of salts are required. Finite-Difference Time-Domain calculations were also employed to study the enhanced near-fields induced around aluminum nanoparticles by a radiating fluorophore, and the effect of such enhanced fields on the fluorescence enhancement observed was discussed.
通过热蒸发将不同厚度的颗粒状铝膜沉积在石英衬底上。这些纳米结构的衬底通过扫描电子显微镜(SEM)进行表征。从SEM图像可以观察到,随着铝厚度的增加,薄膜表面从有节理的逐渐变为光滑的。迄今为止,金属增强荧光(MEF)主要是在可见光-近红外波长区域使用银或金岛膜或粗糙表面观察到的。我们现在表明,使用纳米结构的铝膜在光谱的紫外-蓝光区域也可以增强荧光。本研究选择了两种探针,一种在紫外区域,另一种在蓝光光谱区域。我们观察到在铝纳米结构表面上10纳米旋涂的聚乙烯醇薄膜中,DNA碱基类似物2-氨基嘌呤和香豆素衍生物(7-HC)的发射增加、荧光寿命缩短以及光稳定性增强。荧光增强因子取决于铝膜的厚度,因为形成的纳米结构的尺寸随铝厚度而变化。两种探针在铝纳米结构衬底附近都表现出光稳定性增强,这与较短的寿命一致。我们的初步研究表明,铝纳米结构衬底在MEF应用中可能会有广泛的用途,特别是在紫外-蓝光光谱区域。此外,与用于MEF的常用银胶体基衬底相比,这些铝纳米结构衬底在含有氯盐的缓冲液中非常稳定,从而进一步提高了这些铝基衬底在许多需要高浓度盐的生物测定中的实用性。还采用了时域有限差分计算来研究由辐射荧光团在铝纳米颗粒周围诱导的增强近场,并讨论了这种增强场对观察到的荧光增强的影响。