Chambery Angela, Di Maro Antimo, Parente Augusto
Dipartimento di Scienze della Vita, Seconda Università di Napoli, Caserta, Italy.
Phytochemistry. 2008 Jul;69(10):1973-82. doi: 10.1016/j.phytochem.2008.04.005. Epub 2008 May 29.
Seeds from Phytolacca dioica L. contain at least three N-glycosylated PD-Ss, type 1 ribosome-inactivating proteins (RIPs), which were separated and purified to homogeneity by conventional chromatographic techniques. ESI-Q-TOF mass spectrometry provided the accurate M(r) of native PD-S1 and PD-S3 (30957.1 and 29785.1, respectively) and the major form PD-S2 (30753.8). As the amino acid sequence of PD-S2 was already known, its disulfide pairing was determined and found to be Cys34-Cys262 and Cys88-Cys110. Further structural characterization of PD-S1 and PD-S3 (N-terminal sequence determination up to residue 30, amino acid analysis and tryptic peptide mapping) showed that the three PD-Ss shared the entire protein sequence. To explain the different chromatographic behaviour, their glycosylation patterns were characterized by a fast and sensitive mass spectrometry-based approach, applying a precursor ion discovery mode on a Q-TOF mass spectrometer. A standard plant paucidomannosidic N-glycosylation pattern [Hex(3), HexNAc(2), deoxyhexose(1), pentose(1)] was found for PD-S1 and PD-S2 on Asn120. Furthermore, a glycosylation site carrying only a HexNAc residue was identified on Asn112 in PD-S1 and PD-S3. Finally, considering the two disulfide bridges and the glycan moieties, the experimental M(r) values were in agreement with the mass values calculated from the primary structure. The complete characterization of PD-Ss shows the high potential of mass spectrometry to rapidly characterize proteins, widespread in eukaryotes, differing only in their glycosylation motifs.
垂序商陆的种子含有至少三种N-糖基化的PD-Ss,即1型核糖体失活蛋白(RIPs),通过传统色谱技术将它们分离并纯化至同质。电喷雾-四极杆-飞行时间质谱(ESI-Q-TOF质谱)给出了天然PD-S1和PD-S3的准确相对分子质量(分别为30957.1和29785.1)以及主要形式PD-S2的相对分子质量(30753.8)。由于PD-S2的氨基酸序列已知,确定了其二硫键配对,发现为Cys34-Cys262和Cys88-Cys110。对PD-S1和PD-S3的进一步结构表征(N端序列测定至第30位残基、氨基酸分析和胰蛋白酶肽图谱分析)表明,这三种PD-Ss共享整个蛋白质序列。为了解释不同的色谱行为,采用基于质谱的快速灵敏方法,在Q-TOF质谱仪上应用前体离子发现模式对它们的糖基化模式进行了表征。在Asn120处发现PD-S1和PD-S2具有标准的植物寡甘露糖型N-糖基化模式[己糖(3)、N-乙酰己糖胺(2)、脱氧己糖(1)、戊糖(1)]。此外,在PD-S1和PD-S3的Asn112处鉴定出一个仅携带一个N-乙酰己糖胺残基的糖基化位点。最后,考虑到两个二硫键和聚糖部分,实验相对分子质量值与根据一级结构计算的质量值一致。PD-Ss的完整表征表明,质谱在快速表征真核生物中广泛存在、仅糖基化基序不同的蛋白质方面具有很高的潜力。