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模拟扰动条件下不同营养状态湖泊沉积物的磷释放特征

Phosphorus release characteristics of different trophic lake sediments under simulative disturbing conditions.

作者信息

Wang Shengrui, Jin Xiangcan, Zhao Haichao, Wu Fengchang

机构信息

State Environmental Protection Key Laboratory for Lake Pollution Control, Research Center of Lake Eco-environment, Chinese Research Academy of Environmental Sciences, Chaoyang District, Anwai Da Yangfang, Beijing 100012, China.

出版信息

J Hazard Mater. 2009 Jan 30;161(2-3):1551-9. doi: 10.1016/j.jhazmat.2008.05.004. Epub 2008 May 9.

DOI:10.1016/j.jhazmat.2008.05.004
PMID:18555597
Abstract

The effect of simulative disturbing on phosphorus (P) release characteristics and the differences of the P buffering capacity of different trophic lake sediments were investigated. The magnitudes of the dissolved total phosphorus (DTP), soluble reactive phosphorus (SRP) and dissolved organic phosphorus (DOP) released from the studied sediments increased with the increasing of disturbing intensity. The equilibrium time of the DTP release from the heavily polluted sediments was approximately 16 h, and that from the slightly polluted sediments was 8h. This may be related to the difference of P forms in the different trophic sediments. About 30% of the DTP released from Wuli Lake and Yue Lake was from DOP, about 60% and 50%, respectively, was from Gonghu Lake and East Taihu Lake. DOP was the important fraction of DTP released. The effect of disturbing on P release was related to both disturbing intensity and sediment pollution level. After the disturbing stop, the DTP, SRP and DOP concentrations in the overlying water of the different sediments decreased rapidly within 3, 10 and 3h, respectively, then gradually reached equilibrium at different time for the sediments with different pollution level. The different trophic lake sediments had different P buffering capacity, P buffering capacity of the slightly polluted sediments was lower at the initial lower SRP concentrations and was higher at the initial higher than that of the heavily polluted sediments.

摘要

研究了模拟扰动对不同营养状态湖泊沉积物磷(P)释放特性的影响以及不同营养状态湖泊沉积物磷缓冲能力的差异。研究沉积物释放的溶解总磷(DTP)、溶解性反应磷(SRP)和溶解有机磷(DOP)的量随扰动强度的增加而增加。重污染沉积物中DTP释放的平衡时间约为16小时,轻度污染沉积物中为8小时。这可能与不同营养状态沉积物中磷形态的差异有关。五里湖和月湖释放的DTP中约30%来自DOP,贡湖和太湖东部则分别约为60%和50%。DOP是DTP释放的重要组成部分。扰动对磷释放的影响与扰动强度和沉积物污染程度有关。扰动停止后,不同沉积物上覆水中的DTP、SRP和DOP浓度分别在3小时、10小时和3小时内迅速下降,然后在不同污染程度的沉积物中于不同时间逐渐达到平衡。不同营养状态的湖泊沉积物具有不同的磷缓冲能力,轻度污染沉积物在初始SRP浓度较低时磷缓冲能力较低,而在初始SRP浓度较高时高于重污染沉积物。

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