School of Environmental Science and Technology, Suzhou University of Science and Technology, 99 Xuefu Road, Suzhou, 215009, Jiangsu Province, People's Republic of China.
Environ Sci Pollut Res Int. 2021 Jan;28(2):1837-1849. doi: 10.1007/s11356-020-10602-9. Epub 2020 Aug 28.
The response of the transformation of internal phosphorus (P) to resuspended sediment was investigated in the sediment-water system under different disturbance intensity. The sediments and overlying water were collected from Taihu Lake, a typical shallow lake. The concentrations of particulate P (PP) and dissolved inorganic P (DIP) in the water phase and algal available P (AAP) and P fractions in the sediments and suspended particle characteristics were evaluated in laboratory-simulated experiments. The results show that dissolved oxygen (DO) in the overlying water increased continuously and pH decreased slightly under sediment resuspension. The concentration of ammonia nitrogen (NH-N) showed a distinct decline, indicating that sediment resuspension promotes the penetration of DO into the sediments. It was also favor of the formation of metal oxides and hydroxides, inducing soluble amorphous metal compounds oxidized to insoluble crystalline metal compounds under disturbance condition. This resulted in the increase of refractory P in sediment compared with the static conditions. Sediment resuspension is beneficial to long-term P retention. This can be confirmed by the increase of maximum P adsorption amount (Q) and the decrease of the degree of P saturation (DPS) and equilibrium P concentration (EPC). This is the main explanation of DIP decrease in the overlying water. It is indicating that sediment resuspension not only improves the redox environment in the sediment-water system but also enhances P retention capacity.
研究了不同干扰强度下沉积物-水系统中内部磷(P)转化对再悬浮沉积物的响应。沉积物和上覆水取自典型浅水湖泊太湖。在实验室模拟实验中,评估了水相中颗粒态 P(PP)和溶解无机 P(DIP)的浓度、沉积物和悬浮颗粒特征中的藻类有效 P(AAP)和 P 分数。结果表明,沉积物再悬浮时,上覆水中的溶解氧(DO)持续增加,pH 值略有下降。氨氮(NH-N)浓度明显下降,表明沉积物再悬浮促进了 DO 向沉积物中的渗透。这也有利于金属氧化物和氢氧化物的形成,在干扰条件下,将可溶性无定形金属化合物氧化为不溶性结晶金属化合物。与静态条件相比,这导致沉积物中难溶性 P 的增加。沉积物再悬浮有利于磷的长期保留。上覆水中 DIP 减少可以通过最大磷吸附量(Q)的增加和磷饱和度(DPS)和平衡磷浓度(EPC)的降低来证实。这是 DIP 减少的主要解释。这表明,沉积物再悬浮不仅改善了沉积物-水系统中的氧化还原环境,而且增强了磷的保持能力。