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通过原子台阶低角度阴影法生长的银纳米颗粒阵列中的等离子体共振。

Plasmon resonance in silver nanoparticles arrays grown by atomic terrace low-angle shadowing.

作者信息

Cuccureddu Floriano, Murphy Shane, Shvets Igor V, Porcu Mauro, Zandbergen H W

机构信息

Centre for Research on Adaptive Nanostructures and Nanodevices, School of Physics, Trinity College, Dublin 2, Ireland.

出版信息

Nano Lett. 2008 Oct;8(10):3248-56. doi: 10.1021/nl801600w. Epub 2008 Sep 18.

Abstract

The plasmonic properties of aligned silver nanoparticles grown by atomic terrace low-angle shadowing (ATLAS) were studied by optical transmission spectroscopy. ATLAS is a novel nanofabrication technique that combines the advantages of self-assembly with control of the nanostructure features. The silver nanoarrays were optically characterized and distinct optical responses with strong polarization dependence were obtained indicating the existence of a strong near-field coupling between the particles. We found that different morphologies gave rise to a similar optical response due to the local contributions to the overall response. Numerical model based on discrete dipole approximation was used to give a qualitative insight into the studied phenomena.

摘要

通过光透射光谱法研究了采用原子台阶低角度阴影法(ATLAS)生长的排列银纳米颗粒的等离子体特性。ATLAS是一种新型纳米制造技术,它将自组装的优点与纳米结构特征的控制相结合。对银纳米阵列进行了光学表征,并获得了具有强偏振依赖性的独特光学响应,这表明颗粒之间存在强近场耦合。我们发现,由于对整体响应的局部贡献,不同的形态产生了相似的光学响应。基于离散偶极近似的数值模型被用于对所研究的现象进行定性洞察。

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