Li Y, Balédent V, Barisić N, Cho Y, Fauqué B, Sidis Y, Yu G, Zhao X, Bourges P, Greven M
Department of Physics, Stanford University, Stanford, California 94305, USA.
Nature. 2008 Sep 18;455(7211):372-5. doi: 10.1038/nature07251.
The pseudogap region of the phase diagram is an important unsolved puzzle in the field of high-transition-temperature (high-T(c)) superconductivity, characterized by anomalous physical properties. There are open questions about the number of distinct phases and the possible presence of a quantum-critical point underneath the superconducting dome. The picture has remained unclear because there has not been conclusive evidence for a new type of order. Neutron scattering measurements for YBa(2)Cu(3)O(6+delta) (YBCO) resulted in contradictory claims of no and weak magnetic order, and the interpretation of muon spin relaxation measurements on YBCO and of circularly polarized photoemission experiments on Bi(2)Sr(2)CaCu(2)O(8+delta)(refs 12, 13) has been controversial. Here we use polarized neutron diffraction to demonstrate for the model superconductor HgBa(2)CuO(4+delta) (Hg1201) that the characteristic temperature T* marks the onset of an unusual magnetic order. Together with recent results for YBCO, this observation constitutes a demonstration of the universal existence of such a state. The findings appear to rule out theories that regard T* as a crossover temperature rather than a phase transition temperature. Instead, they are consistent with a variant of previously proposed charge-current-loop order that involves apical oxygen orbitals, and with the notion that many of the unusual properties arise from the presence of a quantum-critical point.
相图中的赝能隙区域是高温超导领域一个重要的未解之谜,其特征是具有反常的物理性质。关于不同相的数量以及超导穹顶下方可能存在的量子临界点,仍存在一些未解决的问题。由于尚未有关于新型有序态的确凿证据,情况一直不明朗。对YBa(2)Cu(3)O(6+δ)(YBCO)的中子散射测量结果存在矛盾,有人声称没有磁有序,也有人称有弱磁有序,而且对YBCO的μ子自旋弛豫测量以及对Bi(2)Sr(2)CaCu(2)O(8+δ)的圆偏振光电子能谱实验(参考文献12、13)的解释一直存在争议。在此,我们利用极化中子衍射证明,对于模型超导体HgBa(2)CuO(4+δ)(Hg1201),特征温度T标志着一种不寻常磁有序的开始。结合最近关于YBCO的结果,这一观察结果证明了这种状态的普遍存在。这些发现似乎排除了将T视为交叉温度而非相变温度的理论。相反,它们与先前提出的涉及顶氧轨道的电荷 - 电流环有序的一个变体一致,并且与许多异常性质源于量子临界点的存在这一观点相符。