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利用光差分透射光谱法研究外延石墨烯中受激狄拉克费米子的超快弛豫

Ultrafast relaxation of excited Dirac fermions in epitaxial graphene using optical differential transmission spectroscopy.

作者信息

Sun Dong, Wu Zong-Kwei, Divin Charles, Li Xuebin, Berger Claire, de Heer Walt A, First Phillip N, Norris Theodore B

机构信息

Center for Ultrafast Optical Science, University of Michigan, Ann Arbor, Michigan 48109-2099, USA.

出版信息

Phys Rev Lett. 2008 Oct 10;101(15):157402. doi: 10.1103/PhysRevLett.101.157402. Epub 2008 Oct 6.

Abstract

We investigate the ultrafast relaxation dynamics of hot Dirac fermionic quasiparticles in multilayer epitaxial graphene using ultrafast optical differential transmission spectroscopy. We observe differential transmission spectra which are well described by interband transitions with no electron-hole interaction. Following the initial thermalization and emission of high-energy phonons, the electron cooling is determined by electron-acoustic phonon scattering, found to occur on the time scale of 1 ps for highly doped layers, and 4-11 ps in undoped layers. The spectra also provide strong evidence for the multilayer structure and doping profile of thermally grown epitaxial graphene on SiC.

摘要

我们使用超快光学差分透射光谱法研究了多层外延石墨烯中热狄拉克费米子准粒子的超快弛豫动力学。我们观察到的差分透射光谱可以通过无电子 - 空穴相互作用的带间跃迁很好地描述。在初始热化和高能声子发射之后,电子冷却由电子 - 声学声子散射决定,发现对于高掺杂层,其发生在1皮秒的时间尺度上,而在未掺杂层中为4 - 11皮秒。这些光谱还为碳化硅上热生长的外延石墨烯的多层结构和掺杂分布提供了有力证据。

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