Sebastian Suchitra E, Harrison N, Sengupta P, Batista C D, Francoual S, Palm E, Murphy T, Marcano N, Dabkowska H A, Gaulin B D
Cavendish Laboratory, University of Cambridge, Madingley Road, Cambridge CB3 0HE, United Kingdom.
Proc Natl Acad Sci U S A. 2008 Dec 23;105(51):20157-60. doi: 10.1073/pnas.0804320105. Epub 2008 Dec 11.
The fractalized Hofstadter butterfly energy spectrum predicted for magnetically confined fermions diffracted by a crystal lattice has remained beyond the reach of laboratory-accessible magnetic fields. We find the geometrically frustrated spin system SrCu(2)(BO(3))(2) to provide a sterling demonstration of a system in which bosons confined by a magnetic and lattice potential mimic the behavior of fermions in the extreme quantum limit, giving rise to a sequence of plateaus at all magnetization m(z)/m(sat) = 1/q ratios 9 > or = q > or = 2 and p/q = 2/9 (m(sat) is the saturation magnetization) in magnetic fields up to 85 T and temperatures down to 29 mK, within the sequence of previously identified plateaus at 1/8, 1/4, and 1/3 of the saturated magnetization. We identify this hierarchy of plateaus as a consequence of confined bosons in SrCu(2)(BO(3))(2) mimicking the high magnetic field fractalization predicted by the Hofstadter butterfly for fermionic systems. Such an experimental realization of the Hofstadter problem for interacting fermions has not been previously achieved in real materials, given the unachievably high magnetic flux densities or large lattice periods required. By a theoretical treatment that includes short-range repulsion in the Hofstadter treatment, stripe-like spin density-modulated phases are revealed in SrCu(2)(BO(3))(2) as emergent from a fluidic fractal spectrum.
对于由晶格衍射的磁约束费米子所预测的分形化霍夫施塔特蝴蝶能谱,一直处于实验室可及磁场范围之外。我们发现几何阻挫自旋系统SrCu₂(BO₃)₂能出色地证明,在该系统中,受磁势和晶格势约束的玻色子在极端量子极限下模仿费米子的行为,在高达85 T的磁场和低至29 mK的温度下,在先前确定的饱和磁化强度的1/8、1/4和1/3的平台序列内,所有磁化强度m(z)/m(sat) = 1/q(9≥q≥2且p/q = 2/9,m(sat)为饱和磁化强度)的比值处都会出现一系列平台。我们将这种平台层级结构确定为SrCu₂(BO₃)₂中受约束的玻色子模仿霍夫施塔特蝴蝶为费米子系统所预测的高磁场分形化的结果。鉴于所需的高得无法实现的磁通密度或大晶格周期,此前在实际材料中尚未实现这种相互作用费米子的霍夫施塔特问题的实验实现。通过一种在霍夫施塔特理论处理中包含短程排斥的理论处理方法,在SrCu₂(BO₃)₂中揭示出条纹状自旋密度调制相是从流体分形谱中涌现出来的。