Lee Ho-Jin, Wang Nick X, Shao Youming, Zheng Jie J
Department of Structural Biology, St Jude Children's Research Hospital, Memphis, TN 38105, USA.
Bioorg Med Chem. 2009 Feb 15;17(4):1701-8. doi: 10.1016/j.bmc.2008.12.060. Epub 2009 Jan 3.
The development of inhibitors of Dishevelled (Dvl) PDZ protein-protein interactions attracts attention due to a possible application in drug discovery and development. Using nuclear magnetic resonance (NMR) spectroscopy, we found that a tripeptide VVV binds to the PDZ domain of Dvl, which is a key component involved in Wnt signaling. Using a computational approach calculating the binding free energy of the complexes of the Dvl PDZ domain and each of the tripeptides VXV (X: any amino acid residue except Pro), we found that a tripeptide VWV had the highest binding affinity. Consistent with the computational result, experimental results showed that the binding of the tripeptide VWV to the Dvl PDZ domain was stronger than that of the tripeptide VVV. The binding affinity of the tripeptide VWV was comparable to that of the organic molecule NSC668036, which was the first identified Dvl PDZ inhibitor. The three-dimensional structure of the complex Dvl1 PDZ/VWV was determined to investigate the role of the energetically favorable W(-1) residue in binding. These interactions were also explored by using molecular dynamic simulation and the molecular mechanics Poisson-Boltzmann surface area method. Taken together, these two tripeptides may be used as modulators of Wnt signaling or as a scaffold to optimize an antagonist for targeting Dvl1 PDZ protein-protein interaction.
由于在药物发现与开发中可能的应用,Dishevelled(Dvl)PDZ蛋白-蛋白相互作用抑制剂的开发备受关注。利用核磁共振(NMR)光谱,我们发现三肽VVV与Dvl的PDZ结构域结合,Dvl是Wnt信号通路中的关键组成部分。通过计算方法计算Dvl PDZ结构域与每种三肽VXV(X:除脯氨酸外的任何氨基酸残基)复合物的结合自由能,我们发现三肽VW的结合亲和力最高。与计算结果一致,实验结果表明三肽VW与Dvl PDZ结构域的结合强于三肽VVV。三肽VW的结合亲和力与首个被鉴定的Dvl PDZ抑制剂有机分子NSC668036相当。确定了复合物Dvl1 PDZ/VW的三维结构,以研究能量上有利的W(-1)残基在结合中的作用。还通过分子动力学模拟和分子力学泊松-玻尔兹曼表面积方法探索了这些相互作用。综上所述,这两种三肽可作为Wnt信号通路的调节剂,或作为优化靶向Dvl1 PDZ蛋白-蛋白相互作用拮抗剂的支架。