Chiu Nan-Fu, Yu Chun, Nien Shou-Yu, Lee Jiun-Haw, Kuan Chieh-Hsiung, Wu Kuang-Chong, Lee Chih-Kung, Lin Chii-Wann
Opt Express. 2007 Sep 3;15(18):11608-15. doi: 10.1364/oe.15.011608.
The effect of coupled mode surface plasmon polaritons (SPPs) on the active emission of a nanostructure grating with organic semiconductor material, Alq(3), on the surface was investigated in this study. We report surface plasmon grating coupled emission (SPGCE) from excited organic layer on metal grating in both organic/metal (2-Layer) and organic/metal/organic/metal (4-Layer) structures. The dispersion relation was obtained from angle-resolved photoluminescence measurement. The resultant emission intensity can have up to 6 times enhancement on the 4- Layer device and the Full-Width Half-Maximum (FWHM) is less than 50 nm. The combination of SPPs on organic/metal interface allows specific directional emission and color appearance of Alq(3) fluorophores. Potential applications of such an active plasmonics with enhanced resonant energy emission due to interactions on the organic/metal nano-grating as biosensor were presented and discussed.
本研究考察了耦合模式表面等离激元极化激元(SPPs)对表面带有有机半导体材料Alq(3)的纳米结构光栅有源发射的影响。我们报道了在有机/金属(双层)和有机/金属/有机/金属(四层)结构中,金属光栅上受激有机层的表面等离激元光栅耦合发射(SPGCE)。通过角分辨光致发光测量获得了色散关系。在四层器件上,所得发射强度可增强至6倍,半高宽(FWHM)小于50 nm。有机/金属界面上的SPPs组合使得Alq(3)荧光团具有特定的定向发射和颜色呈现。本文还介绍并讨论了这种由于有机/金属纳米光栅上的相互作用而具有增强共振能量发射的有源等离子体激元作为生物传感器的潜在应用。