Morimoto Hisao, Katano Kunio, Maekawa Toru
Bio-Nano Electronics Research Center, Toyo University, 2100, Kujirai, Kawagoe, Saitama 350-8585, Japan.
J Chem Phys. 2009 Jul 21;131(3):034905. doi: 10.1063/1.3179687.
We carry out statistical analysis of cluster structures formed by ferromagnetic particles in a dc magnetic field based on a flexible chain model. In the absence of a magnetic field, ferromagnetic particles tend to form ring structures. When a dc magnetic field is applied, the rings are broken into chains if the intensity of the field is sufficiently high since the dipole moment of each particle is aligned in the field direction. We analyze the conditions under which ring-chain structural transitions occur and clarify the dependence of the probabilities of the creation of ring and chain structures on control parameters such as the strength of the dipole-dipole interactive energy between particles, the intensity of the magnetic field and the cluster size.
我们基于柔性链模型对直流磁场中铁磁颗粒形成的团簇结构进行统计分析。在没有磁场的情况下,铁磁颗粒倾向于形成环形结构。当施加直流磁场时,如果磁场强度足够高,环会断裂成链,因为每个颗粒的偶极矩会沿磁场方向排列。我们分析了环 - 链结构转变发生的条件,并阐明了形成环和链结构的概率对诸如颗粒间偶极 - 偶极相互作用能强度、磁场强度和团簇大小等控制参数的依赖性。