Key Laboratory of Regional Climate-Environment Research for Temperate East Asia, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China.
J Hazard Mater. 2009 Dec 30;172(2-3):970-7. doi: 10.1016/j.jhazmat.2009.07.087. Epub 2009 Jul 29.
A continuous observation of organic carbon (OC) and elemental carbon (EC), and PM(10) was conducted at an urban site of Beijing to investigate the characterization of carbonaceous aerosols during spring time. The mean value and standard deviations of OC, EC, PM(10) concentration, and OC/EC ratio were 13.5+/-7.0 microg m(-3), 7.1+/-4.1 microg m(-3), 187.8+/-136.9 microg m(-3), and 2.0+/-0.4, respectively. OC, EC, and total carbonaceous aerosols (TCA) in PM(10) account for 9.3+/-5.7%, 4.7+/-2.7%, and 19.6+/-11.6%, respectively. Good correlations (R(2)=0.7) between OC and EC were observed in spring season. Average OC concentrations are 13.5 microg m(-3) in both daytime and nighttime. Average EC concentrations in daytime (7.4 microg m(-3)) are slightly higher than those in nighttime (6.8 microg m(-3)). Both OC and EC concentrations reach maximum value in morning time (07:30-10:30) due to motor vehicles during the traffic rush hour. PM(10), OC, and EC concentration increase while PM(2.5) concentration, OC/EC ratio, PM(2.5)/PM(10), and TCA/PM(10) ratio decrease in dust period in Beijing. During the observation period, the carbonaceous aerosols from motor vehicle and coal combustion accounted for 76% and 24%, respectively. It shows that the motor vehicle represents the dominant emitter of carbonaceous aerosols associated with PM(10) in Beijing during spring time.
在北京的城市地区进行了一次有机碳 (OC) 和元素碳 (EC) 以及 PM(10) 的连续观测,以研究春季碳质气溶胶的特征。OC、EC、PM(10)浓度和 OC/EC 比的平均值和标准偏差分别为 13.5+/-7.0μg m(-3)、7.1+/-4.1μg m(-3)、187.8+/-136.9μg m(-3)和 2.0+/-0.4。OC、EC 和 PM(10)中的总碳质气溶胶 (TCA) 分别占 9.3+/-5.7%、4.7+/-2.7%和 19.6+/-11.6%。在春季,OC 和 EC 之间存在良好的相关性 (R(2)=0.7)。OC 的平均浓度在白天和夜间均为 13.5μg m(-3)。白天 EC 的平均浓度 (7.4μg m(-3)) 略高于夜间 (6.8μg m(-3))。由于交通高峰期的机动车辆,OC 和 EC 浓度在早晨 (07:30-10:30) 达到最大值。在北京的扬尘期间,PM(10)、OC 和 EC 浓度增加,而 PM(2.5)浓度、OC/EC 比、PM(2.5)/PM(10)和 TCA/PM(10)比降低。在观测期间,机动车和燃煤分别贡献了 76%和 24%的碳质气溶胶。这表明在春季,机动车是北京 PM(10) 相关碳质气溶胶的主要排放源。