Center for Environmental Health Sciences, The University of Montana, Missoula, MT 59812, USA.
Environ Pollut. 2010 Mar;158(3):723-9. doi: 10.1016/j.envpol.2009.10.016. Epub 2009 Nov 7.
During the winters of 2006/2007 and 2007/2008, PM2.5 source apportionment programs were carried out within five western Montana valley communities. Filter samples were analyzed for mass and chemical composition. Information was utilized in a Chemical Mass Balance (CMB) computer model to apportion the sources of PM2.5. Results showed that wood smoke (likely residential woodstoves) was the major source of PM2.5 in each of the communities, contributing from 56% to 77% of the measured wintertime PM2.5. Results of 14C analyses showed that between 44% and 76% of the measured PM2.5 came from a new carbon (wood smoke) source, confirming the results of the CMB modeling. In summary, the CMB model results, coupled with the 14C results, support that wood smoke is the major contributor to the overall PM2.5 mass in these rural, northern Rocky Mountain airsheds throughout the winter months.
在 2006/2007 年和 2007/2008 年的冬季,在蒙大拿州西部的五个山谷社区进行了 PM2.5 源解析计划。对滤膜样本进行了质量和化学成分分析。利用化学质量平衡(CMB)计算机模型中的信息对 PM2.5 的来源进行了分配。结果表明,在每个社区中,木柴燃烧(可能是居民的柴火炉)是 PM2.5 的主要来源,占冬季测量的 PM2.5 的 56%至 77%。14C 分析的结果表明,测量的 PM2.5 中有 44%至 76%来自新的碳(木柴燃烧)源,这证实了 CMB 模型模拟的结果。总之,CMB 模型的结果,加上 14C 的结果,支持了在整个冬季,木柴燃烧是这些农村、落基山北部空气流域中 PM2.5 总质量的主要贡献者。